Ultrafast dynamics of nanoplasmonic stopped-light lasing.

Autor: Wuestner S; The Blackett Laboratory, Department of Physics, Imperial College London, South Kensington Campus, London SW7 2AZ, UK. o.hess@imperial.ac.uk., Pickering T, Hamm JM, Page AF, Pusch A, Hess O
Jazyk: angličtina
Zdroj: Faraday discussions [Faraday Discuss] 2015; Vol. 178, pp. 307-24.
DOI: 10.1039/c4fd00181h
Abstrakt: We study the spatio-temporal dynamics of coherent amplification and lasing in planar gain-enhanced nanoplasmonic structures and show that a singularity in the density of optical states leads to a stopped-light feedback mechanism that allows for cavity-free photonic and surface-plasmon polariton nanolasing. We reveal that in the absence of cavity-induced feedback a phase-locked superposition of a quasi dispersion-free waveguide mode promotes the dynamic formation of a subwavelength lasing mode. Simulations on the basis of a full-time domain Maxwell-Bloch Langevin approach uncover a high spontaneous emission factor β≈0.9 and demonstrate that the stopped-light lasing/spasing mechanism is remarkably robust against interface roughness. Stopped-light surface-plasmon polariton lasing is shown to be stable for gain sections of a width of down to 200 nm but in wider gain structures of the order of 1 μm the dynamics is characterised by spatio-temporally oscillating lasing surface-plasmon polaritons with typical temporal and spatial periods of smaller than 5 fs and smaller than 100 nm. Stopped-light lasing thus provides opportunities for ultrafast nanolasing and the realization of ultra-thin lasing surfaces and offers a new route to ultrafast spasing and cavity-free active quantum plasmonics.
Databáze: MEDLINE