Gold nanoparticle tips for optical field confinement in infrared scattering near-field optical microscopy.

Autor: Wenzel MT; Institute of Applied Photophysics, Technische Universität Dresden, 01062 Dresden, Germany. marc.tobias.wenzel@iapp.de, Härtling T, Olk P, Kehr SC, Grafström S, Winnerl S, Helm M, Eng LM
Jazyk: angličtina
Zdroj: Optics express [Opt Express] 2008 Aug 04; Vol. 16 (16), pp. 12302-12.
DOI: 10.1364/oe.16.012302
Abstrakt: We report on the implementation of metal nanoparticles as probes for scattering and apertureless near-field optical investigations in the mid-infrared (mid-IR) spectral regime. At these wavelengths, an efficient electric-field confinement is necessary and achieved here through a gold metal nanoparticle of 80 nm in diameter (Au80-MNP) acting as the optical antenna. The Au80-MNP is attached to a standard AFM cantilever used as the spatial manipulator. When approached to a sample surface while being illuminated with an infrared beam, the Au80-MNP produces a considerably improved spatial confinement of the electric field compared to an ordinary scattering AFM tip. We demonstrate here the confinement normal to the sample surface by making use of a sample-induced phonon polariton resonance in a ferroelectric lithium niobate sample. Our experimental findings are in very good agreement with the quasistatic dipole model and show improved optical resolution via well-selected antenna particles.
Databáze: MEDLINE