Polymerization transitions in two-dimensional systems of dipolar spheres.

Autor: Stambaugh J; Department of Physics, IPST, and IREAP, University of Maryland, College Park, Maryland 20742, USA., Van Workum K, Douglas JF, Losert W
Jazyk: angličtina
Zdroj: Physical review. E, Statistical, nonlinear, and soft matter physics [Phys Rev E Stat Nonlin Soft Matter Phys] 2005 Sep; Vol. 72 (3 Pt 1), pp. 031301. Date of Electronic Publication: 2005 Sep 15.
DOI: 10.1103/PhysRevE.72.031301
Abstrakt: We investigate the self-organization of dipolar spheres into polymer chains as a fundamental model of the self-assembly of particles having anisotropic interparticle interactions. Our study involves a combination of modeling with vertically vibrated magnetic beads simulating a quasi-two-dimensional fluid at equilibrium and corresponding Monte Carlo simulations of hard spheres with embedded extended dipoles. We find a transition from a gas-like phase to a polymerized phase upon cooling, in accord with the analytic theory of equilibrium polymerization.
Databáze: MEDLINE