Room-temperature ordered photon emission from multiexciton states in single CdSe core-shell nanocrystals.

Autor: Fisher B; Department of Chemistry, Massachusetts Institute of Technology, 77 Massachusetts Avenue, Cambridge, MA 02139, USA., Caruge JM, Zehnder D, Bawendi M
Jazyk: angličtina
Zdroj: Physical review letters [Phys Rev Lett] 2005 Mar 04; Vol. 94 (8), pp. 087403. Date of Electronic Publication: 2005 Mar 03.
DOI: 10.1103/PhysRevLett.94.087403
Abstrakt: We report room-temperature ordered multiphoton emission from multiexciton states of single CdSe(CdZnS) core(-shell) colloidal nanocrystals (NCs) that are synthesized by wet chemical methods. Spectrally and temporally resolved measurements of biexciton and triexciton emission from single NCs are also presented. A simple four level system models the results accurately and provides estimates for biexciton and triexciton radiative lifetimes and quantum yields.
Databáze: MEDLINE