Popis: |
Abstract The functional properties of cuprates are strongly determined by the doping state and carrier density. We present an oxygen doping study of YBa2Cu3O7-δ (YBCO) thin films from underdoped to overdoped state, correlating the measured charge carrier density, $${n}_{\mathrm{H}}$$ n H , the hole doping, p, and the critical current density, $${J}_{c}$$ J c . Our results show experimental demonstration of strong increase of $${J}_{c}$$ J c with $${n}_{\mathrm{H}}$$ n H , up to Quantum Critical Point (QCP), due to an increase of the superconducting condensation energy. The ultra-high $${J}_{c}$$ J c achieved, 90 MA cm−2 at 5 K corresponds to about a fifth of the depairing current, i.e. a value among the highest ever reported in YBCO films. The overdoped regime is confirmed by a sudden increase of $${n}_{\mathrm{H}}$$ n H , associated to the reconstruction of the Fermi-surface at the QCP. Overdoping YBCO opens a promising route to extend the current carrying capabilities of rare-earth barium copper oxide (REBCO) coated conductors for applications. |