Dark brown carbon from wildfires: a potent snow radiative forcing agent?

Autor: Ganesh S. Chelluboyina, Taveen S. Kapoor, Rajan K. Chakrabarty
Jazyk: angličtina
Rok vydání: 2024
Předmět:
Zdroj: npj Climate and Atmospheric Science, Vol 7, Iss 1, Pp 1-10 (2024)
Druh dokumentu: article
ISSN: 2397-3722
DOI: 10.1038/s41612-024-00738-7
Popis: Abstract Deposition of wildfire smoke on snow contributes to its darkening and accelerated snowmelt. Recent field studies have identified dark brown carbon (d-BrC) to contribute 50–75% of shortwave absorption in wildfire smoke. d-BrC is a distinct class of water-insoluble, light-absorbing organic carbon that co-exists in abundance with black carbon (BC) in snow across the world. However, the importance of d-BrC as a snow warming agent relative to BC remains unexplored. We address this gap using aerosol-snow radiative transfer calculations on datasets from laboratory and field measurement. We show d-BrC increases the annual mean snow radiative forcing between 0.6 and 17.9 W m− 2, corresponding to different wildfire smoke deposition scenarios. This is a 1.6 to 2.1-fold enhancement when compared with BC-only deposition on snow. This study suggests d-BrC is an important contributor to snowmelt in midlatitude glaciers, where ~40% of the world’s glacier surface area resides.
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