Autor: |
Gabriel O. Gomes, H. Eugene Stanley, Mariano de Souza |
Jazyk: |
angličtina |
Rok vydání: |
2019 |
Předmět: |
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Zdroj: |
Scientific Reports, Vol 9, Iss 1, Pp 1-8 (2019) |
Druh dokumentu: |
article |
ISSN: |
2045-2322 |
DOI: |
10.1038/s41598-019-48353-4 |
Popis: |
Abstract We use the recently-proposed compressible cell Ising-like model to estimate the ratio between thermal expansivity and specific heat (the Grüneisen parameter Γ s ) in supercooled water. Near the critical pressure and temperature, Γ s becomes significantly sensitive to thermal fluctuations of the order-parameter, a characteristic behavior of pressure-induced critical points. Such enhancement of Γ s indicates that two energy scales are governing the system, namely the coexistence of high- and low-density liquids, which become indistinguishable at the critical point in the supercooled phase. The temperature dependence of the compressibility, sound velocity and pseudo-Grüneisen parameter Γ w are also reported. Our findings support the proposed liquid-liquid critical point in supercooled water in the No-Man’s Land regime, and indicates possible applications of this model to other systems. In particular, an application of the model to the qualitative behavior of the Ising-like nematic phase in Fe-based superconductors is also presented. |
Databáze: |
Directory of Open Access Journals |
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