Phonon Signatures in Photon Correlations
| Autor: | Humphries, Ben S., Green, Dale, Borgh, Magnus O., Jones, Garth A. |
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| Rok vydání: | 2023 |
| Předmět: | |
| Zdroj: | Phys. Rev. Lett. 131, 143601 (2023) |
| Druh dokumentu: | Working Paper |
| DOI: | 10.1103/PhysRevLett.131.143601 |
| Popis: | We show that the second-order, two-time correlation functions for phonons and photons emitted from a vibronic molecule in a thermal bath result in bunching and anti-bunching (a purely quantum effect), respectively. Signatures relating to phonon exchange with the environment are revealed in photon-photon correlations. We demonstrate that cross-correlation functions have a strong dependence on the order of detection giving insight into how phonon dynamics influences the emission of light. This work offers new opportunities to investigate quantum effects in condensed-phase molecular systems. Comment: Author accepted manuscript. 7 pages, 3 figures plus 5 pages of Supplemental material with 7 figures |
| Databáze: | arXiv |
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