Lineshape Analysis of Double-Quantum Multidimensional Coherent Spectra

Autor: Lomsadze, Bachana, Cundiff, Steven T.
Rok vydání: 2020
Předmět:
Zdroj: Phys. Rev. A 102, 043514 (2020)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevA.102.043514
Popis: Double-quantum two-dimensional coherent spectroscopy (MDCS) is a powerful optical method that is used to study optical properties of atomic and complex molecular systems and semiconductor materials. Double-quantum 2D spectra and particularly the peak lineshapes on the spectra can also provide information about many-body interactions. We model 2D spectra by solving the optical Bloch equations and show the effects of correlation between coupled resonances, which also explains the discrepancies between the experimental results reported by multiple groups.
Databáze: arXiv