Engineering the eigenstates of coupled spin-1/2 atoms on a surface

Autor: Yang, Kai, Bae, Yujeong, Paul, William, Natterer, Fabian D., Willke, Philip, Lado, Jose L., Ferrón, Alejandro, Choi, Taeyoung, Fernández-Rossier, Joaquín, Heinrich, Andreas J., Lutz, Christopher P.
Rok vydání: 2017
Předmět:
Zdroj: Phys. Rev. Lett. 119, 227206 (2017)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevLett.119.227206
Popis: Quantum spin networks having engineered geometries and interactions are eagerly pursued for quantum simulation and access to emergent quantum phenomena such as spin liquids. Spin-1/2 centers are particularly desirable because they readily manifest coherent quantum fluctuations. Here we introduce a controllable spin-1/2 architecture consisting of titanium atoms on a magnesium oxide surface. We tailor the spin interactions by atomic-precision positioning using a scanning tunneling microscope (STM), and subsequently perform electron spin resonance (ESR) on individual atoms to drive transitions into and out of quantum eigenstates of the coupled-spin system. Interactions between the atoms are mapped over a range of distances extending from highly anisotropic dipole coupling, to strong exchange coupling. The local magnetic field of the magnetic STM tip serves to precisely tune the superposition states of a pair of spins. The precise control of the spin-spin interactions and ability to probe the states of the coupled-spin network by addressing individual spins will enable exploration of quantum many-body systems based on networks of spin-1/2 atoms on surfaces.
Databáze: arXiv