Hot-Carrier Seebeck Effect: Diffusion and Remote Detection of Hot Carriers in Graphene

Autor: Sierra, J. F., Neumann, I., Costache, M. V., Valenzuela, S. O.
Rok vydání: 2015
Předmět:
Zdroj: Nano Letters, pp 4000-4005, 15 (2015)
Druh dokumentu: Working Paper
DOI: 10.1021/acs.nanolett.5b00922
Popis: We investigate hot carrier propagation across graphene using an electrical nonlocal injection/detection method. The device consists of a monolayer graphene flake contacted by multiple metal leads. Using two remote leads for electrical heating, we generate a carrier temperature gradient that results in a measurable thermoelectric voltage VNL across the remaining (detector) leads. Due to the nonlocal character of the measurement, VNL is exclusively due to the Seebeck effect. Remarkably, a departure from the ordinary relationship between Joule power P and VNL, VNL ~ P, becomes readily apparent at low temperatures, representing a fingerprint of hot-carrier dominated thermoelectricity. By studying VNL as a function of bias, we directly determine the carrier temperature and the characteristic cooling length for hot-carrier propagation, which are key parameters for a variety of new applications that rely on hot-carrier transport.
Databáze: arXiv