Orbital control of effective dimensionality: from spin-orbital fractionalization to confinement in the anisotropic ladder system CaCu2O3

Autor: Bisogni, Valentina, Wohlfeld, Krzysztof, Nishimoto, Satoshi, Monney, Claude, Trinckauf, Jan, Zhou, Kejin, Kraus, Roberto, Koepernik, Klaus, Sekar, Chinnathambi, Strocov, Vladimir, Buechner, Bernd, Schmitt, Thorsten, Brink, Jeroen van den, Geck, Jochen
Rok vydání: 2013
Předmět:
Zdroj: Physical Review Letters 114, 096402 (2015)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevLett.114.096402
Popis: Fractionalization of an electronic quasiparticle into spin, charge and orbital parts is a fundamental and characteristic property of interacting electrons in one dimension. However, real materials are never strictly one-dimensional and the fractionalization phenomena are hard to observe. Here we studied the spin and orbital excitations of the anisotropic ladder material CaCu2O3, whose electronic structure is not one-dimensional. Combining high-resolution resonant inelastic x-ray scattering experiments with theoretical model calculations we show that: (i) spin-orbital fractionalization occurs in CaCu2O3 along the leg direction x through the xz orbital channel as in a 1D system; and (ii) no fractionalization is observed for the xy orbital, which extends in both leg and rung direction, contrary to a 1D system. We conclude that the directional character of the orbital hopping can select different degrees of dimensionality. Using additional model calculations, we show that spin-orbital separation is generally far more robust than the spin-charge separation. This is not only due to the already mentioned selection realized by the orbital hopping, but also due to the fact that spinons are faster than the orbitons.
Comment: 6 pages, 4 figure
Databáze: arXiv