Antiferromagnetic Spin Ice Correlations at (1/2,1/2,1/2) in the Ground State of the Pyrochlore Magnet Tb2Ti2O7

Autor: Fritsch, K., Ross, K. A., Qiu, Y., Copley, J. R. D., Guidi, T., Bewley, R. I., Dabkowska, H. A., Gaulin, B. D.
Rok vydání: 2012
Předmět:
Zdroj: Phys. Rev. B 87, 094410 (2013)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.87.094410
Popis: We present high-resolution single crystal time-of-flight neutron scattering measurements on the candidate quantum spin liquid pyrochlore Tb2Ti2O7 at low temperature and in a magnetic field. At ~70 mK and in zero field, Tb2Ti2O7 reveals diffuse magnetic elastic scattering at (1/2,1/2,1/2) positions in reciprocal space, consistent with short-range correlated regions based on a two-in, two-out spin ice configuration on a doubled conventional unit cell. This elastic scattering is separated from very low-energy magnetic inelastic scattering by an energy gap of ~0.06-0.08 meV. The elastic signal disappears under the application of small magnetic fields and upon elevating temperature. Pinch-point-like elastic diffuse scattering is observed near (1,1,1) and (0,0,2) in zero field at ~70 mK, in agreement with Fennell et al. (Ref. 1), supporting the quantum spin ice interpretation of Tb2Ti2O7.
Comment: 7 pages, 6 figures. Replaced previous version with now published version with corrected figure 5
Databáze: arXiv