Definitive Evidence for Order-by-Quantum-Disorder in Er2Ti2O7

Autor: Savary, Lucile, Ross, Kate A., Gaulin, Bruce D., Ruff, Jacob P. C., Balents, Leon
Rok vydání: 2012
Předmět:
Zdroj: Phys. Rev. Lett. 109, 167201 (2012)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevLett.109.167201
Popis: Here we establish the systematic existence of a U(1) degeneracy of all symmetry-allowed Hamiltonians quadratic in the spins on the pyrochlore lattice, at the mean-field level. By extracting the Hamiltonian of Er2Ti2O7 from inelastic neutron scattering measurements, we then show that the U(1)-degenerate states of Er2Ti2O7 are its classical ground states, and unambiguously show that quantum fluctuations break the degeneracy in a way which is confirmed by experiment. This is the first definitive observation of order-by-disorder in any material. We provide further verifiable consequences of this phenomenon, and several additional comparisons between theory and experiment.
Comment: 4.5 pages, 3 figures, 7.5 pages of Supplemental Material, 8 supplemental figures
Databáze: arXiv