Tuning the two-dimensional electron gas at the LaAlO3/SrTiO3(001) interface by metallic contacts

Autor: López, V. G. Ruiz, Arras, R., Pickett, W. E., Pentcheva, R.
Rok vydání: 2011
Předmět:
Zdroj: Phys. Rev. B 85, 125404 (2012)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.85.125404
Popis: First principles calculations reveal that adding a metallic overlayer on LaAlO3/SrTiO3(001) eliminates the electric field within the polar LaAlO3 film and thus suppresses the thickness-dependent insulator-to-metal transition observed in uncovered films. Independent of the LaAlO3 thickness both the surface and the interface are metallic, with an enhanced interface carrier density relative to LaAlO3/SrTiO3(001) after the metallization transition. Moreover, a monolayer thick metallic Ti-contact exhibits a finite magnetic moment and for a thin SrTiO3-substrate induces a spin-polarized 2D electron gas at the n-type interface due to confinement effects. A diagram of band alignment in M/LaAlO3/SrTiO3(001) and Schottky barriers for M=Ti, Al, and Pt are provided.
Comment: 4 pages, 4 figures, submitted for publication
Databáze: arXiv