Characterization of single-molecule pentanedithiol junctions by inelastic electron tunneling spectroscopy and first-principles calculations

Autor: Arroyo, Carlos R., Frederiksen, Thomas, Rubio-Bollinger, Gabino, Velez, Marisela, Arnau, Andres, Sanchez-Portal, Daniel, Agrait, Nicolas
Rok vydání: 2010
Předmět:
Zdroj: Phys. Rev. B 81, 075405 (2010)
Druh dokumentu: Working Paper
DOI: 10.1103/PhysRevB.81.075405
Popis: We study pentanedithiol molecular junctions formed by means of the break-junction technique with a scanning tunneling microscope at low temperatures. Using inelastic electron tunneling spectroscopy and first-principles calculations, the response of the junction to elastic deformation is examined. We show that this procedure makes a detailed characterization of the molecular junction possible. In particular, our results indicate that tunneling takes place through just a single molecule.
Comment: 5 pages, 4 figures (accepted in Phys. Rev. B)
Databáze: arXiv