Facile Elaboration of Wet Cellulose Film as Catalyst Support of MnOx Nanoparticles for the Catalytic Oxidation of Dyes in Absence of Light
| Autor: | Fernanda F. Camilo, Mary-Lorène Goddard, Marcos A. Bizeto, Ludovic Josien, Samar Hajjar-Garreau, Simona Bennici, Lionel Limousy, Larissa V.F. Oliveira |
|---|---|
| Přispěvatelé: | Institut de Science des Matériaux de Mulhouse (IS2M), Centre National de la Recherche Scientifique (CNRS)-Matériaux et nanosciences d'Alsace (FMNGE), Institut de Chimie du CNRS (INC)-Université de Strasbourg (UNISTRA)-Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Institut National de la Santé et de la Recherche Médicale (INSERM)-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Université de Strasbourg (UNISTRA)-Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Institut National de la Santé et de la Recherche Médicale (INSERM)-Centre National de la Recherche Scientifique (CNRS)-Réseau nanophotonique et optique, Centre National de la Recherche Scientifique (CNRS)-Université de Strasbourg (UNISTRA)-Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Centre National de la Recherche Scientifique (CNRS)-Université de Strasbourg (UNISTRA) |
| Jazyk: | angličtina |
| Rok vydání: | 2021 |
| Předmět: |
Materials science
Catalyst support cellulose film Nanoparticle 02 engineering and technology 010402 general chemistry 01 natural sciences lcsh:TD1-1066 Catalysis chemistry.chemical_compound [CHIM]Chemical Sciences Cellulose indigo carmine dye lcsh:Environmental technology. Sanitary engineering lcsh:TA170-171 General Engineering 021001 nanoscience & nanotechnology Decomposition 6. Clean water 0104 chemical sciences lcsh:Environmental engineering chemistry Catalytic oxidation Chemical engineering Indigo carmine Ionic liquid MnOx nanoparticles 0210 nano-technology catalytic oxidation |
| Zdroj: | Clean Technologies Clean Technologies, MDPI, 2021, 3 (2), pp.288-298. ⟨10.3390/cleantechnol3020016⟩ Clean Technologies, Vol 3, Iss 16, Pp 288-298 (2021) Volume 3 Issue 2 Pages 16-298 |
| ISSN: | 2571-8797 |
| DOI: | 10.3390/cleantechnol3020016⟩ |
| Popis: | International audience; In the present work a remarkably simple procedure for the elaboration of wet cellulose film containing manganese oxide nanoparticles was developed. The films were produced using a mold made by 3D printing using cellulose dissolved in an ionic liquid, which allows the production of thin and homogeneous films of different shapes, types and designs which cannot be made using conventional techniques. Thanks to this possibility, the final catalytic object can be implemented in specific reactors. Manganese oxide nanoparticles were prepared as a colloidal solution by a redox/sol-gel procedure and then deposited on the cellulose films by wet impregnation. The catalytic film obtained was tested in the decomposition of a dye, indigo carmine (IC), in the absence of light. The influence of the pH of the solution on the decomposition rate was investigated. IC total decomposition was measured after 1-h reaction at pH below 3. At pH = 2, no deactivation of the catalyst was observed even after four decomposition cycles. This work provides a new strategy to design cellulose-based catalysts for dye removal from wastewater. |
| Databáze: | OpenAIRE |
| Externí odkaz: |
|