Photoionization spectroscopy of excited states of cold caesium dimers
Autor: | Amodsen Chotia, Maria Allegrini, Daniel Comparat, Olivier Dulieu, Andrea Fioretti, Mireille Aymar, Pierre Pillet, Elena Favilla, Carlo Gabbanini, Matthieu Viteau, Nadia Bouloufa |
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Rok vydání: | 2010 |
Předmět: |
Chemical Physics (physics.chem-ph)
Physics Condensed Matter::Quantum Gases Dye laser Biophysics FOS: Physical sciences Photoionization Condensed Matter Physics Laser law.invention laser cooling law Excited state molecular spectroscopy Physics - Chemical Physics Molecule Physics::Atomic Physics Physical and Theoretical Chemistry Asymptote Atomic physics Ground state Spectroscopy cold molecules Molecular Biology |
Zdroj: | Molecular physics info:cnr-pdr/source/autori:Nadia Bouloufa; Elena Favilla; Matthieu Viteau; Amodsen Chotia; Andrea Fioretti, Carlo Gabbanini; Maria Allegrini; Mireille Aymar; Daniel Comparat; Olivier Dulieu; Pierre Pillet/titolo:Photoionization spectroscopy of excited states of cold caesium dimers/doi:10.1080%2F00268976.2010.495732/rivista:Molecular physics (Print)/anno:2010/pagina_da:2355/pagina_a:2368/intervallo_pagine:2355–2368/volume:108 |
DOI: | 10.1080/00268976.2010.495732 |
Popis: | Photoionization spectroscopy of cold cesium dimers obtained by photoassociation of cold atoms in a magneto-optical trap is reported here. In particular, we report on the observation and on the spectroscopic analysis of all the excited states that have actually been used for efficient detection of cold molecules stabilized in the triplet a^3Sigma_u^+ ground state. They are: the (1)^3Sigma_g^+ state connected to the 6s+6p asymptote, the (2)^3Sigma_g^+ and (2)^3Pi_g states connected to the 6s+5d asymptote and finally the (3)^3Sigma_g^+ state connected to the 6s + 7s asymptote. The detection through these states spans a wide range of laser energies, from 8000 to 16500 cm-1, obtained with different laser dyes and techniques. Information on the initial distribution of cold molecules among the different vibrational levels of the a^3Sigma_u^+ ground state is also provided. This spectroscopic knowledge is important when conceiving schemes for quantum manipulation, population transfer and optical detection of cold cesium molecules. 24 pages, 11 figures. Note: tables are available separately. Accepted in Molecular Physics |
Databáze: | OpenAIRE |
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