Comment on 'Oxygen vacancy-induced magnetic moment in edge-sharing CuO2 chains of Li2CuO2'

Autor: Johannes Richter, Roland Hayn, N. Wizent, Claude Monney, J. Geck, D. Milosavljevic, Satoshi Nishimoto, J. Thar, G. Roth, V. Yushankhai, W. E. A. Lorenz, H. Rosner, A. Hauser, R. O. Kuzian, S.-L. Drechsler, H. Yamaguchi, Rüdiger Klingeler, Liviu Hozoi, Toshimitsu Ito, Thorsten Schmitt, Ravi Yadav, L. Siurakshina, Masaaki Matsuda, Jiří Málek, U. Nitzsche, Steven Johnston
Jazyk: angličtina
Rok vydání: 2018
Předmět:
Zdroj: New journal of physics 20(5), 058001 (2018). doi:10.1088/1367-2630/aac159
Popis: In a recent work devoted to the magnetism of Li$_{2}$CuO$_{2}$, Shu et al. [New J. Phys. 19 (2017) 023026] have proposed a "simplified" unfrustrated microscopic model that differs considerably from the models refined through decades of prior work. We show that the proposed model is at odds with known experimental data, including the reported magnetic susceptibility $\chi(T)$ data up to 550~K. Using an 8$^{\rm th}$ order high-temperature expansion for $\chi(T)$, we show that the experimental data for Li$_{2}$CuO$_{2}$ are consistent with the prior model derived from inelastic neutron scattering (INS) studies. We also establish the $T$-range of validity for a Curie-Weiss law for the real frustrated magnetic system. We argue that the knowledge of the long-range ordered magnetic structure for $T
Comment: 12 pages, 1 figure. Two authors and one reference added as well as slightly changed wording and style (two footnotes added). Short note on the Authors's Reply and Corrigendum is added as well
Databáze: OpenAIRE