Direct observation of spin correlations in an artificial triangular lattice Ising spin system with grazing-incidence small-angle neutron scattering†

Autor: Laura J. Heyderman, Kirill Zhernenkov, Artur Glavic, A Weber, Naëmi Leo, Petai Pip, Sandra H. Skjærvø, Frédéric Mila, Andrew Smerald, Laetitia Philippe
Jazyk: angličtina
Rok vydání: 2021
Předmět:
Zdroj: Nanoscale Horizons
Nanoscale horizons 6(6), 474-481 (2021). doi:10.1039/D1NH00043H
Nanoscale Horizons, 6 (6)
ISSN: 2055-6764
2055-6756
Popis: The triangular lattice with Ising magnetic moments is an archetypical example of geometric frustration. In the case of dipolar-coupled out-of-plane moments, the geometric frustration results in a disordered classical spin-liquid state at higher temperatures while the system is predicted to transition to an anti-ferromagnetic stripe ground state at low temperatures. In this work we fabricate artificial triangular Ising spin systems without and with uniaxial in-plane compression to tune the nature and temperature of the correlations. We probe the energy scale and nature of magnetic correlations by grazing-incidence small-angle neutron scattering. In particular, we apply a newly-developed empirical structure-factor model to describe the measured short-range correlated spin-liquid state, and find good agreement with theoretical predictions. We demonstrate that grazing-incidence neutron scattering on our high-quality samples, in conjunction with detailed modeling of the scattering using the Distorted Wave Born Approximation, can be used to experimentally quantify the spin-liquid-like correlations in highly-frustrated artificial spin systems.
Nanoscale Horizons, 6 (6)
ISSN:2055-6756
ISSN:2055-6764
Databáze: OpenAIRE