Autonomous optimisation of a nanoparticle catalysed reduction reaction in continuous flow

Autor:	Thomas W. Chamberlain, Robert Menzel, Connor J. Taylor, Richard A. Bourne, Alexander F. Massey, Ricardo Labes, Brendan Hall
Rok vydání:	2021
Předmět:	Materials science Kinetic model business.industry Continuous flow Metals and Alloys Nanoparticle General Chemistry Redox Catalysis Surfaces Coatings and Films Electronic Optical and Magnetic Materials Reactor system Materials Chemistry Ceramics and Composites Process engineering business
Zdroj:	Chemical communications (Cambridge, England). 57(40)
ISSN:	1364-548X 1359-7345
Popis:	An automated continuous flow reactor system equipped with inline analysis, was developed and applied in the self-optimisation of a nanoparticle catalysed reaction. The system was used to optimise the experimental conditions of a gold nanoparticle catalysed 4-nitrophenol reduction reaction, towards maximum conversion in under 2.5 hours. The data obtained from this optimisation was then used to generate a kinetic model, allowing us to predict the outcome of the reaction under different conditions. By combining continuous flow nanoparticle synthesis with this approach, the development timeline for these emerging catalysts could be significantly accelerated.
Databáze:	OpenAIRE
Externí odkaz:	https://explore.openaire.eu/search/publication?articleId=doi_dedup___::7175708427d2cf11905b6255a117ec4e https://pubmed.ncbi.nlm.nih.gov/33870978 Zobrazit plný text záznamu