Absence of magnetic ordering and field induced phase diagram in the Gadolinium Aluminium garnet

Autor: E. Lhotel, Christopher S. Knee, Pascale P. Deen, Henrik Jacobsen, O. Florea
Přispěvatelé: Magnétisme et Supraconductivité (MagSup ), Institut Néel (NEEL), Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Niels Bohr Institute [Copenhagen] (NBI), Faculty of Science [Copenhagen], University of Copenhagen = Københavns Universitet (KU)-University of Copenhagen = Københavns Universitet (KU), ESS, Lund, Department of Physics [Oxford], University of Oxford [Oxford], Chalmers, Dept Chem & Chem Engn, SE-41296 Gothenburg, Sweden
Rok vydání: 2018
Předmět:
Zdroj: Physical Review B
Physical Review B, American Physical Society, 2017, 96 (22), pp.220413. ⟨10.1103/PhysRevB.96.220413⟩
ISSN: 2469-9950
2469-9969
DOI: 10.48550/arxiv.1801.02836
Popis: The robustness of spin liquids with respect to small perturbations, and the way magnetic frustration can be lifted by slight changes in the balance between competing magnetic interactions remains a rich and open issue. We address this question through the study of the Gadolinium Aluminium garnet Gd$_3$Al$_5$O$_{12}$, a related compound to the extensively studied Gd$_3$Ga$_5$O$_{12}$. We report on its magnetic properties at very low temperature. We show that despite a freezing at about 300 mK, no magnetic transition is observed, suggesting the presence of a spin liquid state down to the lowest temperatures similarly to Gd$_3$Ga$_5$O$_{12}$, in spite of a larger ratio between exchange and dipolar interactions. Finally, the phase diagram as a function of field and temperature is strongly reminiscent from the one reported in Gd$_3$Ga$_5$O$_{12}$. This study reveals the robust nature of the spin liquid phase for Gd ions on the garnet lattice in stark contrast to Gd ions on the pyrochlore lattice for which a slight perturbation drives the compound into a range of magnetically ordered states.
Comment: 5 pages, 5 figures
Databáze: OpenAIRE