Plasmonic Probe of the Semiconductor to Metal Phase Transition in Vanadium Dioxide
| Autor: | Davon W. Ferrara, Joyeeta Nag, Richard F. Haglund, Evan MacQuarrie, Anthony B. Kaye |
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| Rok vydání: | 2013 |
| Předmět: |
Phase transition
Vanadium Compounds Materials science Analytical chemistry Bioengineering General Materials Science Surface plasmon resonance Plasmon business.industry Mechanical Engineering technology industry and agriculture Oxides General Chemistry Surface Plasmon Resonance Condensed Matter Physics Semiconductor Semiconductors Colloidal gold Atomic electron transition Nanoparticles Optoelectronics Gold Homogeneous broadening business human activities Localized surface plasmon |
| Zdroj: | Nano Letters. 13:4169-4175 |
| ISSN: | 1530-6992 1530-6984 |
| DOI: | 10.1021/nl401823r |
| Popis: | An array of 180 nm diameter gold nanoparticles (NPs) embedded in a thin vanadium dioxide film was used as a nanoscale probe of the thermochromic semiconductor-to-metal transition (SMT) in the VO2. The observed 30% reduction in plasmon dephasing time resulted from the interaction between the localized surface plasmon resonance of the NPs with the 1.4 eV electronic transitions in VO2. The NPs act as nanoantennas probing the SMT; homogeneous broadening of the gold plasmon resonance is observed at the temperatures where electron correlations are strongest in VO2. |
| Databáze: | OpenAIRE |
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