Magnetic ordering and spin-reorientation transitions inTbCo3B2

Autor: Hanania Ettedgui, Mordechai Melamud, El’ad N. Caspi, M. Dubman, Hagai Shaked, Lukas Keller
Rok vydání: 2005
Předmět:
Zdroj: Physical Review B. 72
ISSN: 1550-235X
1098-0121
DOI: 10.1103/physrevb.72.024446
Popis: The magnetic structure of the compound $\mathrm{Tb}{\mathrm{Co}}_{3}{\mathrm{B}}_{2}$ has been studied in the temperature range $1.5\phantom{\rule{0.3em}{0ex}}\mathrm{K}\ensuremath{\leqslant}T\ensuremath{\leqslant}300\phantom{\rule{0.3em}{0ex}}\mathrm{K}$ by means of neutron powder diffraction, magnetization, magnetic ac susceptibility, and heat capacity measurements. The compound is of hexagonal symmetry and is paramagnetic at $300\phantom{\rule{0.3em}{0ex}}\mathrm{K}$, undergoes a magnetic $\mathrm{Co}\text{\ensuremath{-}}\mathrm{Co}$ ordering transition at $\ensuremath{\sim}170\phantom{\rule{0.3em}{0ex}}\mathrm{K}$, and a second magnetic $\mathrm{Tb}\text{\ensuremath{-}}\mathrm{Tb}$ ordering transition at $\ensuremath{\sim}30\phantom{\rule{0.3em}{0ex}}\mathrm{K}$. The latter induces a spin-reorientation transition, in which the magnetic axis rotates from the $c$ axis toward the basal plane. Below this transition a symmetry decrease ($\ensuremath{\gamma}$ magnetostriction) sets in, leading to an orthorhombic distortion of the crystal lattice. The crystal and magnetic structures and interactions and their evolution with temperature are discussed using a microscopic physical model.
Databáze: OpenAIRE