High performance sub-bandgap photodetection via internal photoemission based on ideal metal/2D-material van der Waals Schottky interface

Autor: Songyu Li, Xiaoqing Chen, Xiulong Bao, Feihong Chu, Boxing An, Yongzhe Zhang, Famin Liu, Congya You, Xuhong Li, Jingjie Li, Wenjie Deng, Xiaobo Zhang
Rok vydání: 2021
Předmět:
Zdroj: Nanoscale. 13:16448-16456
ISSN: 2040-3372
2040-3364
DOI: 10.1039/d1nr04770a
Popis: Two-dimensional (2D) materials have been demonstrated to be promising candidates to design high performance photodetectors owing to their strong light-matter interaction. However, the performance of 2D material photodetectors is still unsatisfactory, such as slow response speed due to defects and vulnerable contact interface, which impede their rapid development in the field of optoelectronics. In this paper, we obtained the ideal and large photosensitive van der Waals Schottky interface by the laminating-flipping method. Hence, a fast response speed ( 1012 Jones) are observed on the van der Waals Schottky junction photodiode. More importantly, benefiting from the flat Schottky interface (the roughness ∼0.6 nm), a sub-bandgap light response modulated by the Schottky barrier height (cut-off edge at 1050 nm) has been detected based on the large Au/MoSe2 sensitive Schottky interface internal photoemission. As a result, a universal strategy for the sub-bandgap near-infrared van der Waals Schottky junction detector of 2D materials was obtained.
Databáze: OpenAIRE