Strain Induced Orbital Dynamics Across the Metal Insulator Transition in Thin VO2/TiO2 (001) Films.

Autor: D'Elia, A., Rezvani, S.J., Cossaro, A., Stredansky, M., Grazioli, C., Li, B. W., Zou, C.W., Coreno, M., Marcelli, A.
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Zdroj: Journal of Superconductivity & Novel Magnetism; Aug2020, Vol. 33 Issue 8, p2383-2388, 6p
Abstrakt: VO2 is a strongly correlated material, which undergoes a reversible metal insulator transition (MIT) coupled to a structural phase transition upon heating (T = 67 °C). Since its discovery, the nature of the insulating state has long been debated and different solid-state mechanisms have been proposed to explain its nature: Mott-Hubbard correlation, Peierls distortion, or a combination of both. Moreover, still now, there is a lack of consensus on the interplay between the different degrees of freedom: charge, lattice, orbital, and how they contribute to the MIT. In this manuscript, we will investigate across the MIT the orbital evolution induced by a tensile strain applied to thin VO2 films. The strained films allowed to study the interplay between orbital and lattice degrees of freedom and to clarify MIT properties. [ABSTRACT FROM AUTHOR]
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