Important Elements of Spin-Exciton and Magnon-Exciton Coupling.

Autor: Brennan NJ; Department of Physics, Cornell University, Ithaca, New York 14853, United States., Noble CA; Department of Chemistry and Chemical Biology, Cornell University, Ithaca, New York 14853, United States., Tang J; Department of Chemistry and Chemical Biology, Cornell University, Ithaca, New York 14853, United States., Ziebel ME; Department of Chemistry, Columbia University, New York, New York 10027, United States., Bae YJ; Department of Chemistry and Chemical Biology, Cornell University, Ithaca, New York 14853, United States.
Jazyk: angličtina
Zdroj: ACS physical chemistry Au [ACS Phys Chem Au] 2024 Apr 26; Vol. 4 (4), pp. 322-327. Date of Electronic Publication: 2024 Apr 26 (Print Publication: 2024).
DOI: 10.1021/acsphyschemau.4c00010
Abstrakt: The recent discovery of spin-exciton and magnon-exciton coupling in a layered antiferromagnetic semiconductor, CrSBr, is both fundamentally intriguing and technologically significant. This discovery unveils a unique capability to optically access and manipulate spin information using excitons, opening doors to applications in quantum interconnects, quantum photonics, and opto-spintronics. Despite their remarkable potential, materials exhibiting spin-exciton and magnon-exciton coupling remain limited. To broaden the library of such materials, we explore key parameters for achieving and tuning spin-exciton and magnon-exciton couplings. We begin by examining the mechanisms of couplings in CrSBr and drawing comparisons with other recently identified two-dimensional magnetic semiconductors. Furthermore, we propose various promising scenarios for spin-exciton coupling, laying the groundwork for future research endeavors.
Competing Interests: The authors declare no competing financial interest.
(© 2024 The Authors. Published by American Chemical Society.)
Databáze: MEDLINE