Zobrazeno 1 - 10
of 10
pro vyhledávání: '"Victoria B. F. Custodis"'
Autor:
Patrick Hemberger, Victoria B. F. Custodis, Andras Bodi, Thomas Gerber, Jeroen A. van Bokhoven
Publikováno v:
Nature Communications, Vol 8, Iss 1, Pp 1-9 (2017)
The conversion of lignin by catalytic fast pyrolysis into useful fine chemicals is a promising route to fuel production, however selectivity and conversion are still not optimal. Here, the authors investigate the reaction mechanism by detection of re
Externí odkaz:
https://doaj.org/article/81d27a5cff3647eb811eeb40e593ca63
Autor:
Andras Bodi, Adam J. Trevitt, Victoria B. F. Custodis, Mathias Steglich, Gabriel daSilva, Patrick Hemberger
Publikováno v:
Journal of the American Chemical Society. 139:14348-14351
The meta-xylylene diradical m-C8H8 is a prototypical organic triplet that represents a building block for organic molecule-based magnets and also serves as a model compound for test and refinement of quantum chemical calculations. Flash vacuum pyroly
Autor:
Frédéric Vogel, Gunnar Jeschke, Christian Bährle, Victoria B. F. Custodis, Jeroen A. van Bokhoven
Publikováno v:
ChemSusChem. 9:2397-2403
Lignin from lignocellulosic biomass is a promising source of energy, fuels, and chemicals. The conversion of the polymeric lignin to fuels and chemicals can be achieved by catalytic and noncatalytic pyrolysis. The influence of nonporous silica and ze
Autor:
Victoria B. F. Custodis, Stamatia A. Karakoulia, Jeroen A. van Bokhoven, Kostas S. Triantafyllidis
Publikováno v:
ChemSusChem. 9:1134-1145
Catalytic fast pyrolysis (CFP) of lignin with amorphous mesoporous aluminosilicates catalysts yields a high fraction of aromatics and a relatively low amount of char/coke. The relationship between the acidity and porosity of Al-MCM-41, Al-SBA-15, and
Publikováno v:
Journal of Analytical and Applied Pyrolysis. 115:214-223
This study reveals that catalytic and non-catalytic fast pyrolysis of lignin is influenced by the lignin separation method. Lignin of the same soft- and hardwood source was prepared by the Dioxane-, Klason- and Organsolv-methods and pyrolyzed at diff
Autor:
Thomas Gerber, Jeroen A. van Bokhoven, Victoria B. F. Custodis, Andras Bodi, Patrick Hemberger
Publikováno v:
Nature Communications, 8
Nature Communications, Vol 8, Iss 1, Pp 1-9 (2017)
Nature Communications
Nature Communications, Vol 8, Iss 1, Pp 1-9 (2017)
Nature Communications
Catalytic fast pyrolysis is a promising way to convert lignin into fine chemicals and fuels, but current approaches lack selectivity and yield unsatisfactory conversion. Understanding the pyrolysis reaction mechanism at the molecular level may help t
Publikováno v:
Chemistry (Weinheim an der Bergstrasse, Germany). 23(36)
One of the key challenges in renewable chemical production is the conversion of lignin, especially by fast pyrolysis. The complexity of the lignin pyrolysis process has hindered the elucidation of the mechanism, inhibiting further industrial implemen
Publikováno v:
The Journal of Physical Chemistry B. 118:8524-8531
Fast pyrolysis of lignin is one of the most promising methods to convert the complex and irregular structure of lignin into renewable chemicals and fuel. During pyrolysis the complex set of radical reactions, rearrangements, and eliminations is influ
Autor:
Victoria B. F. Custodis, Frédéric Vogel, Christian Bährle, Gunnar Jeschke, Jeroen A. van Bokhoven
Publikováno v:
ChemSusChem. 7:2022-2029
Lignin pyrolysis is a promising method for the sustainable production of phenolic compounds from biomass. However, detailed knowledge about the radicals involved in this process and their influence on the molecular products is missing. Herein, we rep
Publikováno v:
Catalysis Science & Technology. 4:766
Catalytic fast pyrolysis of lignin was investigated in a pyroprobe microreactor with different catalysts, including (non-)acidic alumina silicates, transition metal oxides, and zeolite-supported transition metals. The results indicate that the select