Zobrazeno 1 - 10
of 65
pro vyhledávání: '"Vassiliy Lubchenko"'
Autor:
Ho Yin Chan, Vassiliy Lubchenko
Publikováno v:
Nature Communications, Vol 10, Iss 1, Pp 1-11 (2019)
Solutions of proteins and other molecules can host puzzling, solute-rich inclusions of mesoscopic dimensions. Here the authors report a mechanism by which mesoscopic clusters can nucleate and ripen, requiring that the solute form long-lived complexes
Externí odkaz:
https://doaj.org/article/373215f46bfa44118246d0282d6295ae
Autor:
Vassiliy Lubchenko
Publikováno v:
Advances in Physics: X, Vol 3, Iss 1 (2018)
Amorphous solids manifest puzzling effects of mysterious degrees of freedom that give rise to a heat capacity and phonon scattering in great excess over what would be expected for a solid that has a unique vibrational ground state. Of particular conc
Externí odkaz:
https://doaj.org/article/ec1c4f60350b4df7af843a767fbc78a1
Autor:
Vassiliy Lubchenko, Yang He
Publikováno v:
The Journal of Chemical Physics. 158:124119
We argue that one can associate a pseudo-time with sequences of configurations generated in the course of classical Monte Carlo simulations for a single-minimum bound state if the sampling is optimal. Hereby, the sampling rates can be, under special
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::23de363d16932b6defbd5b09020b72e4
https://doi.org/10.1063/5.0135479
https://doi.org/10.1063/5.0135479
Publikováno v:
The journal of physical chemistry. B. 125(32)
When a liquid is cooled, progress down the energy landscape is arrested near the glass transition temperature Tg. In principle, lower energy states can be accessed by waiting for further equilibration, but the rough energy landscape of glasses quickl
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::bfe496c277827a9c62258b8a36833f63
https://pubmed.ncbi.nlm.nih.gov/34357766
https://pubmed.ncbi.nlm.nih.gov/34357766
Autor:
Peter G. Wolynes, Vassiliy Lubchenko
Publikováno v:
The journal of physical chemistry. B. 124(38)
We discuss the photon activation of structural relaxations in glassy melts and frozen glasses containing molecules that can photoisomerize. The built-in stress following a photoinduced electronic transition lowers the thermal activation barrier for s
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::370d86c4902ca75cedd976f0a5379402
https://pubmed.ncbi.nlm.nih.gov/32857509
https://pubmed.ncbi.nlm.nih.gov/32857509
Autor:
Peter G. Wolynes, Vassiliy Lubchenko
Publikováno v:
The Journal of Physical Chemistry B. 122:3280-3295
Apart from not having crystallized, supercooled liquids can be considered as being properly equilibrated and thus can be described by a few thermodynamic control variables. In contrast, glasses and other amorphous solids can be arbitrarily far away f
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::d1f3c369089bfd82d027b7c5e8d59c5d
https://doi.org/10.1021/acs.jpcb.7b09553
https://doi.org/10.1021/acs.jpcb.7b09553
Autor:
Arkady A. Kurnosov, Vassiliy Lubchenko
We present a microscopic picture rationalizing the surprisingly steep decrease of the band gap with temperature in insulators, crystalline or otherwise. The gap narrowing largely results from fluctuations of long-wavelength optical phonons---when the
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::70a373bebdae34c5d3e7865c0cef37d7
http://arxiv.org/abs/1809.10773
http://arxiv.org/abs/1809.10773
Publikováno v:
The journal of physical chemistry. B. 122(33)
We determine the electronic density of states for computationally-generated bulk samples of amorphous chalcogenide alloys As$_{x}$Se$_{100-x}$. The samples were generated using a structure-building algorithm reported recently by us ({J. Chem. Phys.}
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::e33b4deb77940c55dfb4def4e639db7a
https://pubmed.ncbi.nlm.nih.gov/30071166
https://pubmed.ncbi.nlm.nih.gov/30071166
Autor:
Ho Yin Chan, Vassiliy Lubchenko
Publikováno v:
Nature Communications, Vol 10, Iss 1, Pp 1-11 (2019)
Nature Communications
Nature Communications
We show systematically that a steady-state ensemble of mesoscopic inclusions of a solute-rich fluid can emerge in liquid solutions well outside the region of stability of the solute-rich phase. Unanticipated by conventional treatments, this type of r
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::b95732008a9112d9486c938ac3a07afe
http://arxiv.org/abs/1806.01134
http://arxiv.org/abs/1806.01134
Autor:
Jacinta C. Conrad, Laurence A. Angel, Mohammad S. Safari, Vassiliy Lubchenko, David H. Hawke, Michael C. Byington, Peter G. Vekilov, Jacob W. McCabe
Protein crystallization is central to understanding of molecular structure in biology, a vital part of processes in the pharmaceutical industry, and a crucial component of numerous disease pathologies. Crystallization starts with nucleation and how n
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::3d0b8a7a4597eaf41a96ba27ecf7e93f