Výsledky vyhledávání - "Thomas L. C. Jansen"

Akademický článek

Interplay between structural hierarchy and exciton diffusion in artificial light harvesting

Autor: Björn Kriete, Julian Lüttig, Tenzin Kunsel, Pavel Malý, Thomas L. C. Jansen, Jasper Knoester, Tobias Brixner, Maxim S. Pshenichnikov

Publikováno v: Nature Communications, Vol 10, Iss 1, Pp 1-11 (2019)

Light-harvesting antennas and efficient energy transfer enable photosynthesis in low light conditions in natural systems. Here the authors resolve exciton properties and the role of structural hierarchy in a model light-harvesting complex by excited-

Externí odkaz: https://doaj.org/article/275547b0c5674c0c966199a185695032

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Akademický článek

Spatially-resolved fluorescence-detected two-dimensional electronic spectroscopy probes varying excitonic structure in photosynthetic bacteria

Autor: Vivek Tiwari, Yassel Acosta Matutes, Alastair T. Gardiner, Thomas L. C. Jansen, Richard J. Cogdell, Jennifer P. Ogilvie

Publikováno v: Nature Communications, Vol 9, Iss 1, Pp 1-10 (2018)

2D electronic spectroscopy enables a spatially-averaged view of the electronic structure of a heterogeneous system. Here, the authors extend it to sub-micron resolution and ~106 times better sensitivity, to resolve spatially varying excitonic structu

Externí odkaz: https://doaj.org/article/7149b8f4130d415293f0e8b256e98c51

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The effect of caesium alloying on the ultrafast structural dynamics of hybrid organic-inorganic halide perovskites

Autor: Nathaniel P. Gallop, Junzhi Ye, Gregory M. Greetham, Thomas L. C. Jansen, Linjie Dai, Szymon J. Zelewski, Rakesh Arul, Jeremy J. Baumberg, Robert L. Z. Hoye, Artem A. Bakulin

Publikováno v: Journal of Materials Chemistry A, 10(42), 22408-22418. ROYAL SOC CHEMISTRY

Hybrid inorganic-organic perovskites have attracted considerable attention over recent years as promising processable electronic materials. In particular, the rich structural dynamics of these ‘soft’ materials has become a subject of investigatio

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::5c8e6d6742ef9a95a35ee4d1104ec7d2
https://hdl.handle.net/11370/1ec17164-4f71-47e3-85ce-788e4c9d1f6e

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Modeling the Effect of Disorder in the Two-Dimensional Electronic Spectroscopy of Poly-3-hexyltiophene in an Organic Photovoltaic Blend: A Combined Quantum/Classical Approach

Autor: Elisa Palacino-González, Thomas L. C. Jansen

Publikováno v: Journal of Physical Chemistry C, 127(14), 6793-6801. AMER CHEMICAL SOC

We introduce a first-principles model of the 12-mer poly-3-hexyltiophene (P3HT) polymer system in the realistic description of an organic photovoltaic blend environment. We combine Molecular Dynamics (MD) simulations of a thin-film blend of P3HT and

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::0b6867ce5b93754bca76cff50678d1e7
https://research.rug.nl/en/publications/ba00f4b9-181b-4a96-b632-ef9486db1b5a

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Ultrafast Excitation Energy Transfer Dynamics in the LHCII–CP29–CP24 Subdomain of Plant Photosystem II

Autor: Thanh Nhut Do, Hoang Long Nguyen, Parveen Akhtar, Kai Zhong, Thomas L. C. Jansen, Jasper Knoester, Stefano Caffarri, Petar H. Lambrev, Howe-Siang Tan

Publikováno v: The Journal of Physical Chemistry Letters, 13(19). AMER CHEMICAL SOC
Journal of Physical Chemistry Letters
Journal of Physical Chemistry Letters, 2022, 13 (19), pp.4263-4271. ⟨10.1021/acs.jpclett.2c00194⟩

We measure the two-dimensional electronic spectra of the LHCII(M)-CP29-CP24 complex in photosystem II (PSII) and provide the first study of the ultrafast excitation energy transfer (EET) processes of an asymmetric and native light-harvesting assembly

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::9e87b0beb17b367b79683014feaaebe3
https://doi.org/10.1021/acs.jpclett.2c00194

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An efficient time-domain implementation of the multichromophoric Förster resonant energy transfer method

Autor: Kai Zhong, Hoang Long Nguyen, Thanh Nhut Do, Howe-Siang Tan, Jasper Knoester, Thomas L. C. Jansen

Publikováno v: Journal of Chemical Physics, 158(6). AMER INST PHYSICS

The excitation energy transfer (EET) process for photosynthetic antenna complexes consisting of subunits, each comprised of multiple chromophores, remains challenging to describe. The multichromophoric Förster resonance energy transfer theory is a p

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::8ec3067738df58e295770002235354eb
https://research.rug.nl/en/publications/cae8563c-a5df-4a5d-8470-29eecffa4da6

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Manifestation of Hydrogen Bonding and Exciton Delocalization on the Absorption and Two-Dimensional Electronic Spectra of Chlorosomes

Autor: Vesna Erić, Xinmeng Li, Lolita Dsouza, Sean K. Frehan, Annemarie Huijser, Alfred R. Holzwarth, Francesco Buda, G. J. Agur Sevink, Huub J. M. de Groot, Thomas L. C. Jansen

Publikováno v: Journal of Physical Chemistry B, 127(5), 1097-1109. AMER CHEMICAL SOC
Journal of physical chemistry B, 127(5), 1097-1109. American Chemical Society
Journal of Physical Chemistry B, 127(5), 1097-1109

Chlorosomes are supramolecular aggregates that contain thousands of bacteriochlorophyll molecules. They perform the most efficient ultrafast excitation energy transfer of all natural light-harvesting complexes. Their broad absorption band optimizes l

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::ef6ad0bd6b5cda5ac21bc395253ea1c2
http://hdl.handle.net/10852/101460

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Structural Disorder as the Origin of Optical Properties and Spectral Dynamics in Squaraine Nano-Aggregates

Autor: Robin Bernhardt, Marìck Manrho, Jennifer Zablocki, Lukas Rieland, Arne Lützen, Manuela Schiek, Klaus Meerholz, Jingyi Zhu, Thomas L. C. Jansen, Jasper Knoester, Paul H. M. van Loosdrecht

Publikováno v: Journal of the American Chemical Society, 144(42). AMER CHEMICAL SOC

In contrast to regular J- and H-aggregates, thin film squaraine aggregates usually have broad absorption spectra containing both J-and H-like features, which are favorable for organic photovoltaics. Despite being successfully applied in organic photo

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::7e7aebe1b9f458de021fcaa0af44f6d5
https://research.rug.nl/en/publications/4446a22c-5df9-45b9-ad85-ad93b77652cd

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Quantum-Classical Simulation of Molecular Motors Driven Only by Light

Autor: Thomas L. C. Jansen, Atreya Majumdar

Publikováno v: JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 12(23), 5512-5518. AMER CHEMICAL SOC
The Journal of Physical Chemistry Letters

Molecular motors that exhibit controlled unidirectional rotation provide great prospects for many types of applications including nanorobotics. Existing rotational motors have two key components: photoisomerisation around a pi-bond followed by a ther

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::30583d579c76accbbe95d4c50db2c32d
https://research.rug.nl/en/publications/74635f8d-0cff-4442-8a81-d925381677b5

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An Exciton Dynamics Model of Bryopsis corticulans Light-Harvesting Complex II

Autor: Thanh Nhut Do, Howe-Siang Tan, Jian Ren Shen, Petar H. Lambrev, Jasper Knoester, Thomas L. C. Jansen, Hoang Long Nguyen, Wenda Wang, Parveen Akhtar

Publikováno v: Journal of Physical Chemistry B, 125(4), 1134-1143. AMER CHEMICAL SOC

Bryopsis corticulans is a marine green macroalga adapted to the intertidal environment. It possesses siphonaxanthin-binding light-harvesting complexes of photosystem II (LHCII) with spectroscopic properties markedly different from the LHCII in plants

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::86667277aa92228efc398d9eadc8bfe5
https://doi.org/10.1021/acs.jpcb.0c10634

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