Zobrazeno 1 - 10
of 25
pro vyhledávání: '"Stephen C. Jensen"'
Autor:
Michael R. Wasielewski, Stephen C. Jensen, Dick T. Co, Emily A. Weiss, Ryan M. Young, Yilei Wu, Matthew D. Krzyaniak, Edward J. Dale, Nicolaas A. Vermeulen, Kedy Edme, J. Fraser Stoddart
Publikováno v:
Journal of the American Chemical Society. 138:6163-6170
Time-resolved optical spectroscopies reveal multielectron transfer from the biexcitonic state of a CdS quantum dot to an adsorbed tetracationic compound cyclobis(4,4'-(1,4-phenylene) bipyridin-1-ium-1,4-phenylene-bis(methylene)) (ExBox(4+)) to form b
Publikováno v:
The Journal of Physical Chemistry C. 118:29242-29251
Photo-oxidation of formaldehyde is important because it is an atmospheric pollutant and a possible intermediate along the pathway for CO2 reduction to methanol. By using temperature-programmed reaction spectroscopy as the main tool, we demonstrate th
Publikováno v:
ACS Nano. 8:2826-2837
This paper describes the surface composition-dependent binding of the dichloride salt of methyl viologen (MV2+) to CdS quantum dots (QDs) enriched, to various degrees, with either Cd or S at the surface. The degree of enrichment is controlled synthet
Autor:
Stephen C. Jensen, Cynthia M. Friend
Publikováno v:
Topics in Catalysis. 56:1377-1388
Defect sites in titania have a substantial effect on many thermal and photochemical reactions. Three common types of defects are titanium interstitials, oxygen vacancies and oxygen adatoms—all of which can react with organic molecules adsorbed on t
Publikováno v:
Journal of the American Chemical Society. 135:574-577
Methyl formate is produced from the photo-oxidation of methanol on preoxidized TiO(2)(110). We demonstrate that two consecutive photo-oxidation steps lead to methyl formate using mass spectrometry and scanning tunneling microscopy. The first step in
Publikováno v:
Journal of the American Chemical Society. 138(5)
This paper describes the use of cadmium sulfide quantum dots (CdS QDs) as visible-light photocatalysts for the reduction of nitrobenzene to aniline through six sequential photoinduced, proton-coupled electron transfers. At pH 3.6-4.3, the internal qu
Publikováno v:
The Journal of Physical Chemistry C. 116:21508-21513
Carboxylic acid moieties are used to anchor organic dyes to TiO2 in many applications; therefore, their structure, distribution on the surface, and thermal and photochemical stability are extremely important. Herein, we investigate the thermal and ph
Publikováno v:
ACS Nano. 6:2925-2930
We demonstrate the one-dimensional confinement of weakly bound butyrophenone molecules between strongly bound complexes formed via reaction with oxygen on TiO(2)(110). Butyrophenone weakly bound to Ti rows through the carbonyl oxygen diffuses freely
Publikováno v:
ACS Nano. 5:834-843
We report the first visualization of a reactive intermediate formed from coupling two molecules on a surface-a diolate formed from benzaldehyde coupling on TiO(2)(110). The diolate, imaged using scanning tunneling microscopy (STM), is reduced to gase
Publikováno v:
ACS Nano. 1:22-29
This paper describes a low-temperature scanning tunneling microscopy (STM) study of a simple thioether, dibutyl sulfide, on a Cu{111} surface. The literature is full of data about thiol-based monolayers; however, relatively little is known about thio