Intermediate-spin iron(IV)-oxido species with record reactivity

Autor: Comba, Peter, Nunn, George, Scherz, Frederik, Walton, Paul H

The nonheme iron(IV)-oxido complex trans-N3-[(L1)FeIVO(Cl)]+, where L1 is a derivative of the tetradentate bispidine 2,4-di(pyridine-2-yl)-3,7-diazabicyclo[3.3.1]nonane-1-one, has an S = 1 electronic ground state and is the most reactive nonheme iron

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https://eprints.whiterose.ac.uk/185085/1/Author_accepted_ms_before_corrections.pdf

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Intermediate-spin iron(IV)-oxido species with record reactivity.

Autor: Comba P; Universität Heidelberg, Anorganisch-Chemisches Institut, INF 270, D-69120 Heidelberg, Germany. peter.comba@aci.uni-heidelberg.de.; Universität Heidelberg, Interdisziplinäres Zentrum für Wissenschaftliches Rechnen (IWR), Germany., Nunn G; Department of Chemistry, University of York, Heslington, YORK, YO10 5DD, UK., Scherz F; Universität Heidelberg, Anorganisch-Chemisches Institut, INF 270, D-69120 Heidelberg, Germany. peter.comba@aci.uni-heidelberg.de., Walton PH; Department of Chemistry, University of York, Heslington, YORK, YO10 5DD, UK.

Publikováno v: Faraday discussions [Faraday Discuss] 2022 May 18; Vol. 234 (0), pp. 232-244. Date of Electronic Publication: 2022 May 18.