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We identify many larger organics as products of electrochemical CO2 reduction in high-current GDEs – most interestingly, C4 and C5 isomers. The analysis of selectivity trends allows for deduction of general hypotheses to build a detailed mechanism.
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=od_______109::84eb987aec0e0f6b8434e66b5d4f8fe9
https://www.repository.cam.ac.uk/handle/1810/347445
https://www.repository.cam.ac.uk/handle/1810/347445
Autor:
Chitre A; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK.; Cambridge Centre for Advanced Research and Education in Singapore, CARES Ltd. 1 CREATE Way, CREATE Tower #05-05, Singapore, 138602, Singapore.; Institute of Materials Research and Engineering, Agency for Science, Technology and Research (A*STAR), Singapore, 138634, Singapore., Querimit RCM; Institute of Materials Research and Engineering, Agency for Science, Technology and Research (A*STAR), Singapore, 138634, Singapore.; School of Chemistry, Chemical Engineering and Biotechnology, Nanyang Technological University, Singapore, 637459, Singapore., Rihm SD; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK.; Cambridge Centre for Advanced Research and Education in Singapore, CARES Ltd. 1 CREATE Way, CREATE Tower #05-05, Singapore, 138602, Singapore., Karan D; Cambridge Centre for Advanced Research and Education in Singapore, CARES Ltd. 1 CREATE Way, CREATE Tower #05-05, Singapore, 138602, Singapore., Zhu B; BASF Advanced Chemicals Co. Ltd., No. 300, Jiang Xin Sha Road, Pudong, Shanghai, 200137, China., Wang K; BASF Advanced Chemicals Co. Ltd., No. 300, Jiang Xin Sha Road, Pudong, Shanghai, 200137, China., Wang L; BASF Advanced Chemicals Co. Ltd., No. 300, Jiang Xin Sha Road, Pudong, Shanghai, 200137, China., Hippalgaonkar K; Institute of Materials Research and Engineering, Agency for Science, Technology and Research (A*STAR), Singapore, 138634, Singapore. kedar@ntu.edu.sg.; School of Materials Science and Engineering, Nanyang Technological University, Singapore, 639798, Singapore. kedar@ntu.edu.sg., Lapkin AA; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK. aal35@cam.ac.uk.; Cambridge Centre for Advanced Research and Education in Singapore, CARES Ltd. 1 CREATE Way, CREATE Tower #05-05, Singapore, 138602, Singapore. aal35@cam.ac.uk.
Publikováno v:
Scientific data [Sci Data] 2024 Jul 03; Vol. 11 (1), pp. 728. Date of Electronic Publication: 2024 Jul 03.
Autor:
Rihm SD; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philipppa Fawcett Drive, Cambridge, CB3 0AS, United Kingdom; Department of Chemical & Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, 117585, Singapore., Tan YR; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore., Ang W; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore., Hofmeister M; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philipppa Fawcett Drive, Cambridge, CB3 0AS, United Kingdom; Department of Chemical & Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, 117585, Singapore., Deng X; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore., Laksana MT; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore., Quek HY; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore., Bai J; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philipppa Fawcett Drive, Cambridge, CB3 0AS, United Kingdom., Pascazio L; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore., Siong SC; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore., Akroyd J; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philipppa Fawcett Drive, Cambridge, CB3 0AS, United Kingdom; CMCL Innovations, Sheraton House, Cambridge, CB3 0AX, United Kingdom., Mosbach S; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philipppa Fawcett Drive, Cambridge, CB3 0AS, United Kingdom; CMCL Innovations, Sheraton House, Cambridge, CB3 0AX, United Kingdom., Kraft M; CARES, Cambridge Centre for Advanced Research and Education in Singapore, 1 CREATE Way, CREATE Tower, #05-05, 138602, Singapore; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philipppa Fawcett Drive, Cambridge, CB3 0AS, United Kingdom; CMCL Innovations, Sheraton House, Cambridge, CB3 0AX, United Kingdom; School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, 637459, Singapore; The Alan Turing Institute, 2QR, John Dodson House, 96 Euston Rd, London, NW1 2DB, United Kingdom. Electronic address: mk306@cam.ac.uk.
Publikováno v:
SLAS technology [SLAS Technol] 2024 Jun; Vol. 29 (3), pp. 100135. Date of Electronic Publication: 2024 May 03.
Autor:
Bai J; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK., Mosbach S; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK.; Cambridge Centre for Advanced Research and Education in Singapore (CARES), 1 Create Way, CREATE Tower, #05-05, Singapore, 138602, Singapore., Taylor CJ; Astex Pharmaceuticals, 436 Cambridge Science Park Milton Road, Cambridge, CB4 0QA, UK.; Innovation Centre in Digital Molecular Technologies, Yusuf Hamied Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge, CB2 1EW, UK.; Faculty of Engineering, University of Nottingham, University Park, Nottingham, NG7 2RD, UK., Karan D; Cambridge Centre for Advanced Research and Education in Singapore (CARES), 1 Create Way, CREATE Tower, #05-05, Singapore, 138602, Singapore., Lee KF; CMCL Innovations, Sheraton House, Cambridge, CB3 0AX, UK., Rihm SD; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK.; Cambridge Centre for Advanced Research and Education in Singapore (CARES), 1 Create Way, CREATE Tower, #05-05, Singapore, 138602, Singapore., Akroyd J; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK.; Cambridge Centre for Advanced Research and Education in Singapore (CARES), 1 Create Way, CREATE Tower, #05-05, Singapore, 138602, Singapore., Lapkin AA; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK.; Cambridge Centre for Advanced Research and Education in Singapore (CARES), 1 Create Way, CREATE Tower, #05-05, Singapore, 138602, Singapore.; Innovation Centre in Digital Molecular Technologies, Yusuf Hamied Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge, CB2 1EW, UK., Kraft M; Department of Chemical Engineering and Biotechnology, University of Cambridge, Philippa Fawcett Drive, Cambridge, CB3 0AS, UK. mk306@cam.ac.uk.; Cambridge Centre for Advanced Research and Education in Singapore (CARES), 1 Create Way, CREATE Tower, #05-05, Singapore, 138602, Singapore. mk306@cam.ac.uk.; School of Chemical and Biomedical Engineering, Nanyang Technological University, 62 Nanyang Drive, 637459, Singapore, Singapore. mk306@cam.ac.uk.; The Alan Turing Institute, London, NW1 2DB, UK. mk306@cam.ac.uk.
Publikováno v:
Nature communications [Nat Commun] 2024 Jan 23; Vol. 15 (1), pp. 462. Date of Electronic Publication: 2024 Jan 23.