Výsledky vyhledávání

Bioinspired Trinuclear Copper Catalyst for Water Oxidation with a Turnover Frequency up to 20000 s–1

Autor: Ming-Tian Zhang, Rong-Zhen Liao, Qi-Fa Chen, Ze-Yu Cheng

Publikováno v: Journal of the American Chemical Society. 143:19761-19768

Solar-powered water splitting is a dream reaction for constructing an artificial photosynthetic system for producing solar fuels. Natural photosystem II is a prototype template for research on artificial solar energy conversion by oxidizing water int

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::ca5727e4961d09609a8057cdb2d97955
https://doi.org/10.1021/jacs.1c08078

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Buffer anion effects on water oxidation catalysis: The case of Cu(III) complex

Autor: Qi-Fa Chen, Hao-Yi Du, Ming-Tian Zhang

Publikováno v: Chinese Journal of Catalysis. 42:1338-1344

Water oxidation is the bottleneck of artificial photosynthesis. Since the first ruthenium-based molecular water oxidation catalyst, the blue dimer, was reported by Meyer's group in 1982, catalysts based on transition metals have been widely employed

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::8eb0fc0c1e8e53c0cb9adf61667f6431
https://doi.org/10.1016/s1872-2067(20)63729-9

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Identifying Metal-Oxo/Peroxo Intermediates in Catalytic Water Oxidation by In Situ Electrochemical Mass Spectrometry

Autor: Xianhao Zhang, Qi-Fa Chen, Jintao Deng, Xinyu Xu, Jirui Zhan, Hao-Yi Du, Zhengyou Yu, Meixian Li, Ming-Tian Zhang, Yuanhua Shao

Publikováno v: Journal of the American Chemical Society. 144(39)

Molecular catalysis of water oxidation has been intensively investigated, but its mechanism is still not yet fully understood. This study aims at capturing and identifying key short-lived intermediates directly during the water oxidation catalyzed by

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::5bc5ad411941d74af41faaf64f71816d
https://pubmed.ncbi.nlm.nih.gov/36149317

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Redox‐Active Ligand Assisted Catalytic Water Oxidation by a Ru IV =O Intermediate

Autor: Fei Xie, Qi-Fa Chen, Ming-Tian Zhang, Yu-Hua Guo, Jing Shi

Publikováno v: Angewandte Chemie International Edition. 59:4000-4008

Water splitting is one of the most promising solutions for storing solar energy in a chemical bond. Water oxidation is still the bottleneck step because of its inherent difficulty and the limited understanding of the O-O bond formation mechanism. Mol

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::7373f34f5457806fbb919da9edca36de
https://doi.org/10.1002/anie.201910614

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Bioinspired Trinuclear Copper Catalyst for Water Oxidation with a Turnover Frequency up to 20000 s

Autor: Qi-Fa, Chen, Ze-Yu, Cheng, Rong-Zhen, Liao, Ming-Tian, Zhang

Publikováno v: Journal of the American Chemical Society. 143(47)

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=pmid________::8c94ebbd22dfa97164795ff0950c956b
https://pubmed.ncbi.nlm.nih.gov/34793144

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Bioinspired molecular clusters for water oxidation

Autor: Qi-Fa Chen, Ming-Tian Zhang, Yu-Hua Guo, Yi-Han Yu

Publikováno v: Coordination Chemistry Reviews. 448:214164

Water oxidation (2 H2O → 4H+ + 4 e- + O2) is a key step in utilization of solar energy for producing hydrogen of artificial photosynthetic system. Inspired by the oxygen evolution complex (OEC) in PSII, molecular catalysts are extensively studied a

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::906d3a839d6d62e981e5ab11f17acd02
https://doi.org/10.1016/j.ccr.2021.214164

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