Zobrazeno 1 - 10
of 13
pro vyhledávání: '"Pieter J. Smeets"'
Autor:
Edward I. Solomon, Julia S. Woertink, Robert A. Schoonheydt, Michael A. Vance, Pieter J. Smeets, Marijke H. Groothaert, Bert F. Sels
Publikováno v:
Proceedings of the National Academy of Sciences. 106:18908-18913
Driven by the depletion of crude oil, the direct oxidation of methane to methanol has been of considerable interest. Promising low-temperature activity of an oxygen-activated zeolite, Cu-ZSM-5, has recently been reported in this selective oxidation a
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::bd3ee92aab77efa064f92415e9232b1a
https://doi.org/10.1073/pnas.0910461106
https://doi.org/10.1073/pnas.0910461106
Publikováno v:
Applied Catalysis B: Environmental. 84:505-513
Co–ZSM-5 prepared via different methods with Co/Al ratios ranging from 0.03 to 0.83 are investigated in both the direct N 2 O decomposition and the selective catalytic reduction (SCR) of NO with CH 4 . UV–vis and H 2 -TPR are used to get an insig
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_________::8a0216c22d4b29d570668b2159ade76c
https://doi.org/10.1016/j.apcatb.2008.05.002
https://doi.org/10.1016/j.apcatb.2008.05.002
Autor:
Emiel J. M. Hensen, Robert A. Schoonheydt, Hugo Leeman, Robert M. van Teeffelen, Pieter J. Smeets, Bert F. Sels
Publikováno v:
Journal of Catalysis, 256(2), 183-191. Academic Press Inc.
The catalytic decomposition of N2O was studied over Cu-containing zeolites with different Cu loadings and framework topologies (MFI, MOR, FER, BEA, and FAU). The influence of NO, O2, and H2O on the rate of N2O decomposition was investigated in detail
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::26ff55bcbe1b12c57e5b470663d0b919
https://doi.org/10.1016/j.jcat.2008.03.008
https://doi.org/10.1016/j.jcat.2008.03.008
Publikováno v:
Catalysis Today. 110:303-309
An extensive series of 30 Cu exchanged zeolites and Cu impregnated silicas and aluminas have been tested in their capacities to stabilize the bis(μ-oxo)dicopper core. This core shows a remarkably activity towards methane, as it selectively hydroxyla
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_________::d728eb01dbfddb5e16ff6c8d40968886
https://doi.org/10.1016/j.cattod.2005.09.028
https://doi.org/10.1016/j.cattod.2005.09.028
Autor:
Ryan G. Hadt, Robert A. Schoonheydt, Bert F. Sels, Pieter Vanelderen, Pieter J. Smeets, Edward I. Solomon
The present work highlights recent advances in elucidating the methane oxidation mechanism of inorganic Cu-ZSM-5 biomimic and in identifying the reactive intermediates that are involved. Such molecular understanding is important in view of upgrading
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::749b3a08c4b3fc30d82c6949be92b20e
https://europepmc.org/articles/PMC3593946/
https://europepmc.org/articles/PMC3593946/
Autor:
Matthew T. Kieber-Emmons, Julia S. Woertink, David E. Heppner, Pieter J. Smeets, Jake W. Ginsbach, Christian H. Kjaergaard, Li Tian, Edward I. Solomon
Publikováno v:
ChemInform. 42
Cu/O2 intermediates in biological, homogeneous, and heterogeneous catalysts exhibit unique spectral features that reflect novel geometric and electronic structures that make significant contributions to reactivity. This review considers how the respe
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_________::1fcaa49a7edb42f2f08a793e2777bf98
https://doi.org/10.1002/chin.201118189
https://doi.org/10.1002/chin.201118189
Autor:
David E. Heppner, Jake W. Ginsbach, Edward I. Solomon, Matthew T. Kieber-Emmons, Julia S. Woertink, Li Tian, Christian H. Kjaergaard, Pieter J. Smeets
Publikováno v:
Faraday discussions. 148
Cu/O2 intermediates in biological, homogeneous, and heterogeneous catalysts exhibit unique spectral features that reflect novel geometric and electronic structures that make significant contributions to reactivity. This review considers how the respe
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::4acdc044ddacdb970c70bbcc2f08bb5a
https://pubmed.ncbi.nlm.nih.gov/21322475
https://pubmed.ncbi.nlm.nih.gov/21322475
Autor:
Julia S. Woertink, Pieter J. Smeets, Ryan G. Hadt, Robert A. Schoonheydt, Pieter Vanelderen, Edward I. Solomon, Bert F. Sels
Publikováno v:
Journal of the American Chemical Society. 132(42)
The reactive oxidizing species in the selective oxidation of methane to methanol in oxygen activated Cu-ZSM-5 was recently defined to be a bent mono(μ-oxo)dicopper(II) species, [Cu(2)O](2+). In this communication we report the formation of an O(2)-p
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::5608e2da33bbaa2821c5f00a224b8552
https://pubmed.ncbi.nlm.nih.gov/20923156
https://pubmed.ncbi.nlm.nih.gov/20923156
Publikováno v:
Inorganic chemistry. 49(8)
Zeolites containing transition-metal ions (TMIs) often show promising activity as heterogeneous catalysts in pollution abatement and selective oxidation reactions. In this paper, two aspects of research on the TMIs Cu, Co, and Fe in zeolites are disc
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::43ee628b980d3c69986a9037dd8e2234
https://pubmed.ncbi.nlm.nih.gov/20380459
https://pubmed.ncbi.nlm.nih.gov/20380459
Autor:
Gustaaf Van Tendeloo, Stuart Turner, An Philippaerts, Pieter J. Smeets, Filip de Clippel, Pierre Jacobs, Metin Bulut, Sabine Paulussen, Bert F. Sels, Oleg I. Lebedev, Hilde Poelman
Publikováno v:
Journal of catalysis
JOURNAL OF CATALYSIS
JOURNAL OF CATALYSIS
Different zeolites were tested for selective removal of methyl elaidate ( trans isomer) from an equimolar mixture with methyl oleate ( cis isomer). Sorption experiments of the geometric isomers show that only ZSM-5 samples with reduced Al content in
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::5974d3f2b3acf230b5331e10f1fe99af
https://hdl.handle.net/10067/824350151162165141
https://hdl.handle.net/10067/824350151162165141