Zobrazeno 1 - 10
of 208
pro vyhledávání: '"Peter J Chupas"'
Autor:
Renfeng Li, Luhong Wang, Liangliang Li, Tony Yu, Haiyan Zhao, Karena W. Chapman, Yanbin Wang, Mark L. Rivers, Peter J. Chupas, Ho-kwang Mao, Haozhe Liu
Publikováno v:
Scientific Reports, Vol 7, Iss 1, Pp 1-7 (2017)
Abstract In situ high energy X-ray pair distribution function (PDF) measurements, microtomography and reverse Monte Carlo simulations were used to characterize the local structure of liquid gallium up to 1.9 GPa. This pressure range includes the well
Externí odkaz:
https://doaj.org/article/508b00fc4b2e43e5b54b03146120d69d
Autor:
Michelle L. Beauvais, Bryan A. Sanchez Monserrate, Tianshi Feng, Renkun Chen, Ping Liu, Peter J. Chupas, Karena W. Chapman
Publikováno v:
Journal of Applied Crystallography. 55:258-264
Probing short-lived reaction species is challenging owing to the need for both high signal-to-noise ratio, which can require long measurement time, and fast time resolution. Here, a novel in situ sample environment is presented that decouples time re
Publikováno v:
ACS Materials Letters. 3:698-703
Short-lived reaction intermediates play a critical role in mediating material synthesis. Such short-lived species often elude characterization because of the mismatch between the time scale of meas...
Autor:
Antonin Grenier, Philip J. Reeves, Karena W. Chapman, Clare P. Grey, Kamila M. Wiaderek, Hao Liu, Katharina Märker, Peter J. Chupas, Ieuan D. Seymour
Publikováno v:
Journal of the American Chemical Society. 142:7001-7011
Substituted Li-layered transition-metal oxide (LTMO) electrodes such as LixNiyMnzCo1-y-zO2 (NMC) and LixNiyCo1-y-zAlzO2 (NCA) show reduced first cycle Coulombic efficiency (90-87% under standard cycling conditions) in comparison with the archetypal L
Autor:
Peter G. Khalifah, Karena W. Chapman, Gabrielle E. Kamm, Hao Liu, Peter J. Chupas, Antonin Grenier, Gerard S. Mattei, Zhuo Li, Liang Yin, Monty R. Cosby
Publikováno v:
Journal of Applied Crystallography. 53:133-139
Operando studies that probe how electrochemical reactions propagate through a battery provide valuable feedback for optimizing the electrode architecture and for mitigating reaction heterogeneity. Transmission-geometry depth-profiling measurements ca
Autor:
Michelle L. Beauvais, Karena W. Chapman, Antonin Grenier, Daniel O'Nolan, Haiyan Zhao, Zhihengyu Chen, Mark A. Newton, Peter J. Chupas, Tina M. Nenoff
Publikováno v:
Chemical Science, 12 (41)
Chemical Science
Chemical Science
Unraveling the complex, competing pathways that can govern reactions in multicomponent systems is an experimental and technical challenge. We outline and apply a novel analytical toolkit that fully leverages the synchronicity of multimodal experiment
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::164b035162e821f1c96808ae8ef92372
https://hdl.handle.net/20.500.11850/509885
https://hdl.handle.net/20.500.11850/509885
Autor:
Marco Di Michiel, Saeed Kazemiabnavi, Gavin Vaughan, Karena W. Chapman, Antonin Grenier, Katsuyo Thornton, Peter J. Chupas, Hao Liu, Bryant J. Polzin
Publikováno v:
ACS Applied Materials & Interfaces. 11:18386-18394
In composite battery electrode architectures, local limitations in ionic and electronic transport can result in nonuniform energy storage reactions. Understanding such reaction heterogeneity is important to optimizing battery performance, including r
Autor:
Karena W. Chapman, Daniel O'Nolan, Peter J. Chupas, Yevgeny Rakita, Rebecca D. McAuliffe, Simon J. L. Billinge, Gabriel M. Veith
Publikováno v:
Journal of the American Chemical Society. 142(44)
We achieve a target material state by using a recursive algorithm to control the material reaction based on real-time feedback on the system chemistry from in situ X-ray absorption spectroscopy. Without human intervention, the algorithm controlled O
Autor:
Karena W. Chapman, David Montiel, Daniel O'Nolan, Allison Wustrow, Katsuyo Thornton, Guanglong Huang, Chia-Hao Liu, Gabrielle E. Kamm, Paul K. Todd, Peter J. Chupas, Antonin Grenier, Simon J. L. Billinge, Gia Thinh Tran, James R. Neilson
Publikováno v:
J Appl Crystallogr
Temperature is a ubiquitous environmental variable used to explore materials structure, properties and reactivity. This article reports a new paradigm for variable-temperature measurements that varies the temperature continuously across a sample such
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::abbb982d4b3ff8b30a3ff3f0cdb01a8a
https://europepmc.org/articles/PMC7312153/
https://europepmc.org/articles/PMC7312153/
Autor:
Mahalingam Balasubramanian, Karena W. Chapman, Olaf J. Borkiewicz, Peter J. Chupas, Anna J. Lehner, Claudia Göbel, Ram Seshadri, Megan M. Butala, Kamila M. Wiaderek, Shiri Arnon, Vicky V. T. Doan-Nguyen, Margaret A. Lumley
Publikováno v:
The Journal of Physical Chemistry C. 122:24559-24569
The drive toward high energy density alternatives to Li-ion batteries has led to great interest in energy storage materials not inherently constrained by the capacity limits of the currently employed intercalation electrode materials. Among the alter