Výsledky vyhledávání - "Monika Brady"

Consanguineous Families of Coordinated Carbon: A ReC4Re Assembly That Is Isolable in Three Oxidation States, Including Crystallographically Characterized ReC⋮CC⋮CRe and +ReCCCCRe+ Adducts and a Radical Cation in Which Charge Is Delocalized between Rhenium Termini

Autor: Atta M. Arif, J. A. Gladysz, Weiqing Weng, Marlis Böhme, Jeffery W. Seyler, Yuanlin Zhou, Monika Brady, Angelo J. Amoroso, Gernot Frenking

Publikováno v: Journal of the American Chemical Society. 119:775-788

Reaction of (η5-C5Me5)Re(NO)(PPh3)(C⋮CH) and Cu(OAc)2 (1.5 equiv, 80 °C, pyridine) gives the orange-brown ReC4Re complex (η5-C5Me5)Re(NO)(PPh3)(C⋮CC⋮C)(Ph3P)(ON)Re(η5-C5Me5) (2, 88%) as a 50:50 diastereomer mixture. Crystallization affords

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::478646a48a18da8587c066ea12577459
https://doi.org/10.1021/ja9631817

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A Step-Growth Approach to Metal-Capped One-Dimensional Carbon Allotropes: Syntheses of C12, C16, and C20μ-Polyynediyl Complexes

Autor: Roman Dembinski, Tamás Bartik, Berit Bartik, Monika Brady, John A. Gladysz

Publikováno v: Angewandte Chemie International Edition in English. 35:414-417

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::2ef684c2b7a293d3263d0e7a2734f20b
https://doi.org/10.1002/anie.199604141

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Synthesis, Structure, and Redox Chemistry of Heteropolymetallic Carbon Complexes with MC2M', MC4M', and MC4M'C4M Linkages. Transmetalations of Lithiocarbon Complexes (.eta.5-C5Me5)Re(NO)(PPh3)(C.tplbond.CLi) and (.eta.5-C5Me5)Re(NO)(PPh3)(C.tplbond.CC.tplbond.CLi)

Autor: John A. Gladysz, Berit Bartik, Atta M. Arif, Monika Brady, Tamás Bartik, Weiqing Weng, James A. Ramsden

Publikováno v: Journal of the American Chemical Society. 117:11922-11931

One major objective has been the preparation of compounds in which sp carbon chains span two metals, L{sub n}M(C){sub x}M`L`{sub n`} (I). There are now many examples of such C{sub 2} complexes. However, higher homologs remain much less well explored.

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::69d17f7b22d94966a8117bde72831986
https://doi.org/10.1021/ja00153a014

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Synthesis, Structure, and Reactivity of Chiral RheniumN-Pyrrolyl Complexes Regiochemistry of Electrophilic Addition and Unprecedented Rearrangements to Carbon-Ligated Species

Autor: Charles L. Mayne, Atta M. Arif, Luke J. Alvey, John A. Gladysz, Todd J. Johnson, Monika Brady

Publikováno v: Chemistry - A European Journal. 1:294-303

Reaction of [{Re}(OTf)] (1; {Re} — (η5-C5H5)Re(NO)(PPh3) and potassium pyrrolide gives the N-pyrrolyl complex 2, 88%). Reactions of 2 with (CF3CO)2O/N(C2H5)3 and CH3O2CC=CCO2CH3 give 3- and 2-substituted pyrrolyl complexes respectively (3, R/R′

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::679532bed475d13f3c343259a5e20ad6
https://doi.org/10.1002/chem.19950010506

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Durch schrittweises Kettenwachstum zu eindimensionalen Kohlenstoffallotropen mit terminalen Metallkomplexfragmenten; Synthese von C12-, C16- und C20-μ-Polyindiylkomplexen

Autor: Monika Brady, Tamás Bartik, John A. Gladysz, Roman Dembinski, Berit Bartik

Publikováno v: Angewandte Chemie. 108:467-469

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::ea918485e3d35069eeb5d884362ba894
https://doi.org/10.1002/ange.19961080415

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New families of coordinated carbon: oxidative coupling and cross-coupling of a transition metal butadiynyl complex to bimetallic M–CCCCCCCC–M and M–CCCCCC–M adducts

Autor: John A. Gladysz, Weiqing Weng, Monika Brady

Publikováno v: J. Chem. Soc., Chem. Commun.. :2655-2656

[(η5-C5Me5)Re(NO)(PPh3)(CCCCCCCC)(Ph3P)(ON)Re(η5-C5Me5)] and [(η5-C5Me5)Re(NO)(PPh3)(CCCCCC)-(Ph3P)(ON)Re(η5-C5Me5)], which contain the longest chains of elemental carbon tethered between two transition metals to date, are prepared by Cu(OAc)2 co

Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::580f5c2d7bda3154a014a1ef31853546
https://doi.org/10.1039/c39940002655

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