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Aryl isocyanates are introduced as comonomers for ring-opening copolymerization (ROCOP) with epoxides. Informed by studies of reaction kinetics, we show that divergent sequence selectivity for AB- and ABB-type copolymers can be achieved with a single
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=doi_dedup___::44b77f427a3daab2697dc58eaf7701db
Publikováno v:
Nature chemistry. 12(3)
Given the important role played by 2-hydroxybiaryls in organic, medicinal and materials chemistry, concise methods for the synthesis of this common motif are extremely valuable. In seeking to extend the lexicon of synthetic chemists in this regard, w
Autor:
Henrik Junge, Matthias Beller, Nils Rockstroh, Steffen Fischer, Mark Jurrat, Alastair J. J. Lennox, Shu-Ping Luo, Ralf Ludwig
Publikováno v:
Lennox, A J J, Fischer, S, Jurrat, M, Luo, S P, Rockstroh, N, Junge, H, Ludwig, R & Beller, M 2016, ' Copper-Based Photosensitisers in Water Reduction : A More Efficient in Situ Formed System and Improved Mechanistic Understanding ', Chemistry-A European Journal, vol. 22, no. 4, pp. 1233-1238 . https://doi.org/10.1002/chem.201503812
The reduction of water has been achieved through a non-noble-metal-based homogeneous catalyst system that is formed in situ. Optimisation of the ligand quantities increased catalyst turnover numbers compared to preformed complexes. Mechanistic studie