Zobrazeno 1 - 10
of 65
pro vyhledávání: '"Malerz, Sebastian"'
Autor:
Trinter, Florian, Inhester, Ludger, Püttner, Ralph, Malerz, Sebastian, Thürmer, Stephan, Marchenko, Tatiana, Piancastelli, Maria Novella, Simon, Marc, Winter, Bernd, Hergenhahn, Uwe
Publikováno v:
J. Chem. Phys. 160, 194503 (2024)
We present a combined experimental and theoretical investigation of the radiationless decay spectrum of an O 1s double core hole in liquid water. Our experiments were carried out using liquid-jet electron spectroscopy from cylindrical microjets of no
Externí odkaz:
http://arxiv.org/abs/2402.06419
Autor:
Mudryk, Karen, Lee, Chin, Tomaník, Lukáš, Malerz, Sebastian, Trinter, Florian, Hergenhahn, Uwe, Neumark, Daniel M., Slavíček, Petr, Bradforth, Stephen, Winter, Bernd
Publikováno v:
J. Am. Chem. Soc. 146, 16062-16075 (2024)
Site-specific information on how adenosine triphosphate in the aqueous phase (ATP$_{(aq)}$) interacts with magnesium (Mg$^{2+}_{(aq)}$) is a prerequisite to understanding its complex biochemistry. To gather such information, we apply liquid-jet photo
Externí odkaz:
http://arxiv.org/abs/2306.05352
Autor:
Pugini, Michele, Credidio, Bruno, Walter, Irina, Malerz, Sebastian, Trinter, Florian, Stemer, Dominik, Hergenhahn, Uwe, Meijer, Gerard, Wilkinson, Iain, Winter, Bernd, Thürmer, Stephan
Publikováno v:
Chem. Sci. 14, 9574-9588 (2023)
The recent application of concepts from condensed-matter physics to photoelectron spectroscopy (PES) of volatile, liquid-phase systems has enabled the measurement of electronic energetics of liquids on an absolute scale. Particularly, vertical ioniza
Externí odkaz:
http://arxiv.org/abs/2303.08188
Autor:
He, Lanhai, Tomaník, Lukáš, Malerz, Sebastian, Trinter, Florian, Trippel, Sebastian, Belina, Michal, Slavíček, Petr, Winter, Bernd, Küpper, Jochen
Publikováno v:
J. Phys. Chem. Lett. 14, 10499-10508 (2023)
Solvent interactions, particularly hydration, are vital in chemical and biochemical systems. Model systems unveil microscopic details of such interactions. We uncover a specific hydrogen-bonding motif of the biomolecular building block indole (C$_8$H
Externí odkaz:
http://arxiv.org/abs/2205.08217
Autor:
Schewe, H. Christian, Credidio, Bruno, Ghrist, Aaron M., Malerz, Sebastian, Ozga, Christian, Knie, André, Haak, Henrik, Meijer, Gerard, Winter, Bernd, Osterwalder, Andreas
We present chemical kinetics measurements of the luminol oxydation chemiluminescence reaction at the interface between two aqueous solutions, using liquid jet technology. Free-flowing iquid microjets are a relatively recent development that has found
Externí odkaz:
http://arxiv.org/abs/2201.05008
Autor:
Pohl, Marvin, Malerz, Sebastian, Trinter, Florian, Lee, Chin, Kolbeck, Claudia, Wilkinson, Iain, Thürmer, Stephan, Neumark, Daniel M., Nahon, Laurent, Powis, Ivan, Meijer, Gerard, Winter, Bernd, Hergenhahn, Uwe
Publikováno v:
Phys. Chem. Chem. Phys. 24, 8081-8092 (2022)
We present an experimental X-ray photoelectron circular dichroism (PECD) study of liquid fenchone at the C 1s edge. A novel setup to enable PECD measurements on a liquid microjet [Malerz et al., Rev. Sci. Instrum., 2022, 93, 015101] was used. For the
Externí odkaz:
http://arxiv.org/abs/2201.02277
Autor:
Malerz, Sebastian, Haak, Henrik, Trinter, Florian, Stephansen, Anne B., Kolbeck, Claudia, Pohl, Marvin, Hergenhahn, Uwe, Meijer, Gerard, Winter, Bernd
Publikováno v:
Rev. Sci. Instrum. 93, 015101 (2022)
We present a unique experimental design that enables the measurement of photoelectron circular dichroism (PECD) from chiral molecules in aqueous solution. The effect is revealed from the intensity difference of photoelectron emission into a backward-
Externí odkaz:
http://arxiv.org/abs/2109.14365
Autor:
Credidio, Bruno, Pugini, Michele, Malerz, Sebastian, Trinter, Florian, Hergenhahn, Uwe, Wilkinson, Iain, Thürmer, Stephan, Winter, Bernd
Publikováno v:
Phys. Chem. Chem. Phys. 24, 1310-1325 (2022)
Recent advancement in quantitative liquid-jet photoelectron spectroscopy enables the accurate determination of the absolute-scale electronic energetics of liquids and species in solution. Our major objective is the determination of the absolute lowes
Externí odkaz:
http://arxiv.org/abs/2107.06161
Autor:
Thürmer, Stephan, Malerz, Sebastian, Trinter, Florian, Hergenhahn, Uwe, Lee, Chin, Neumark, Daniel M., Meijer, Gerard, Winter, Bernd, Wilkinson, Iain
Publikováno v:
Chem. Sci. 12, 10558-10582 (2021)
The absolute-scale electronic energetics of liquid water and aqueous solutions, both in the bulk and at associated interfaces, are the central determiners of water-based chemistry. However, such information is generally experimentally inaccessible. W
Externí odkaz:
http://arxiv.org/abs/2104.01630
Autor:
Malerz, Sebastian, Trinter, Florian, Hergenhahn, Uwe, Ghrist, Aaron, Ali, Hebatallah, Nicolas, Christophe, Saak, Clara-Magdalena, Richter, Clemens, Hartweg, Sebastian, Nahon, Laurent, Lee, Chin, Goy, Claudia, Neumark, Daniel M., Meijer, Gerard, Wilkinson, Iain, Winter, Bernd, Thürmer, Stephan
Publikováno v:
Phys. Chem. Chem. Phys. 23, 8246-8260 (2021)
We report on the effects of electron collision and indirect ionization processes, occurring at photoexcitation and electron kinetic energies well below 30 eV on the photoemission spectra of liquid water. We show that the nascent photoelectron spectru
Externí odkaz:
http://arxiv.org/abs/2102.10082