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pro vyhledávání: '"King C. Lai"'
Autor:
Dapeng Jing, Ann Lii-Rosales, King C Lai, Qiang Li, Jaeyoun Kim, Michael C Tringides, James W Evans, Patricia A Thiel
Publikováno v:
New Journal of Physics, Vol 22, Iss 5, p 053033 (2020)
We use a variety of experimental techniques to characterize Cu clusters on bulk MoS _2 formed via physical vapor deposition of Cu in ultrahigh vacuum, at temperatures ranging from 300 K to 900 K. We find that large facetted clusters grow at elevated
Externí odkaz:
https://doaj.org/article/40909a3909174727a69c66eff2983cf0
Publikováno v:
The Journal of Chemical Physics. 158:104102
Shape stability is key to avoiding degradation of performance for metallic nanocrystals synthesized with facetted non-equilibrium shapes to optimize properties for catalysis, plasmonics, and so on. Reshaping of facetted nanocrystals is controlled by
Autor:
Yong Han, King C. Lai, Chia-Kuang Tsung, Wenyu Huang, Benjamin P. Williams, James W. Evans, Minda Chen
Publikováno v:
ACS Nano. 14:8551-8561
Stability against reshaping of metallic fcc nanocrystals synthesized with tailored far-from-equilibrium shapes is key to maintaining optimal properties for applications such as catalysis. Yet Arrhenius analysis of experimental reshaping kinetics, and
Publikováno v:
The Journal of Physical Chemistry C. 124:7492-7499
Au(111) surfaces play a central role in many applications, yet studies of fundamental aspects of their dynamics are limited. Thus, using Scanning Tunneling Microscopy (STM) at 300 K, we analyze the coarsening of first-layer 2D Au islands directly on
Publikováno v:
ACS applied materialsinterfaces.
Metallic nanocrystals (NCs) can be synthesized with tailored nonequilibrium shapes to enhance desired properties, e.g., octahedral fcc metal NCs optimize catalytic activity associated with {111} facets. However, maintenance of optimized properties re
Autor:
King C. Lai, Yong Han, Michael C. Tringides, James W. Evans, Ann Lii-Rosales, Patricia A. Thiel
Publikováno v:
Surface Science. 685:48-58
We have generated precise values for several key energies that are relevant to Cu-graphene or Cu-graphite systems. Such systems may find technological applications that range from graphene synthesis, to condensation heat transfer, to electrical conta
Autor:
King C. Lai, Wenyu Huang, Patricia A. Thiel, Yong Han, Peter M. Spurgeon, James W. Evans, Da-Jiang Liu
Publikováno v:
Chemical Reviews. 119:6670-6768
Self-assembly of supported 2D or 3D nanocrystals (NCs) by vacuum deposition and of 3D NCs by solution-phase synthesis (with possible subsequent transfer to a support) produces intrinsically nonequilibrium systems. Individual NCs can have far-from-equ
Publikováno v:
The Journal of Physical Chemistry C. 123:9528-9537
Synthesis of nanocrystals yields polydisperse distributions, which not only implies a distribution of nanocrystal sizes but also of shapes. Noting that the synthesis products often reflect kinetic effects and may not reflect minimum energy states, we
Autor:
Michael C. Tringides, Kai-Tak Wan, Cai-Zhuang Wang, Scott Julien, James W. Evans, Dapeng Jing, King C. Lai, Patricia A. Thiel, Yong Han, Ann Lii-Rosales
Publikováno v:
Nanoscale. 13(3)
Encapsulation of metal nanoparticles just below the surface of a prototypical layered material, graphite, is a recently discovered phenomenon. These encapsulation architectures have potential for tuning the properties of two-dimensional or layered ma