Zobrazeno 1 - 10
of 40
pro vyhledávání: '"Karl‐Ludwig Kompa"'
Publikováno v:
Angewandte Chemie International Edition. 48:4162-4165
Wie Miniatur-Schneeballe wirken neutrale Cluster aus einigen tausend Molekulen: Treffen sie mit ausreichender Geschwindigkeit auf eine Oberflache, so konnen sie von dieser Biomolekule wie Insulin ablosen. Weil die Cluster wahrend und nach dem Aufpral
Publikováno v:
Chemical Physics. 347:531-545
The feasibility of controlled ultrafast pumping in the mid IR and the probe of the subsequent intramolecular dynamics is illustrated for vibrational excitation of the two metal carbonyls W(CO) 6 and Mn(CO) 5 Br in solution. Pumping and probing is per
Publikováno v:
Chemical Physics Letters. 421:523-528
The enhancement of vibrational modes by phase-shaped femtosecond laser pulses is studied under resonant and non-resonant conditions in an open loop coherent control experiment using non-linear Raman spectroscopy. Applying multipulse sequences matchin
Publikováno v:
The European Physical Journal D. 30:379-392
We report a new approach to intense-field photoionization that is based on the ad hoc assumption that m photons of energy $E_{\rm ph}$ arriving within a typical electronic response time are effectively equivalent to a single photon of energy $mE_{\rm
Publikováno v:
Chemical Physics Letters. 392:156-161
Femtosecond mid-infrared excitation of room temperature W(CO) 6 / n -hexane solutions resonant with the T 1u CO-stretching mode transfers vibrational population to at least v =6. The population distribution in levels v =0 to v =5 was measured by tran
Autor:
Christoph Gebhardt, Vladimir V. Gridin, Israel Schechter, Anna Tomsic, Hartmut Schröder, Karl-Ludwig Kompa
Publikováno v:
International Journal of Mass Spectrometry. 232:1-7
Cluster impact induced charge separation was studied with neat and mixed clusters of SO2 and H2O impinging at hyperthermal velocities on a SiOx target held at different temperatures. At 750 K, impact of SO2 clusters produces positively and negatively
Publikováno v:
Journal of Raman Spectroscopy. 35:934-938
Femtosecond time-resolved degenerate four-wave mixing (DFWM) spectroscopy with ultrashort laser pulses was applied to probe pure rotational Raman transitions of the H2 molecule. Owing to the broad bandwidth of the sub-20 fs pulse, several pure rotati
Publikováno v:
The Journal of Chemical Physics. 119:6314-6323
The fragmentation dynamics of (H2O)1032 clusters colliding with a repulsive surface at incident velocities of 1753 m/s and 2909 m/s, corresponding to kinetic energies of 0.5 and 1.5 times the cluster binding energy, has been examined in a classical m
Autor:
Karl-Ludwig Kompa, Jake S. Yeston, C. Bradley Moore, Detlev Proch, Marcus Motzkus, Thomas Witte, Werner Fuß, Lars Windhorn
Publikováno v:
The Journal of Chemical Physics. 119:641-645
Gaseous diazomethane (CH2N2) has been irradiated with femtosecond laser pulses tuned to the CNN asymmetric stretch at 2100 cm−1 in the mid-infrared. Laser-induced fluorescence detection of 1CH2 [537 nm, b1B1(0 16 0)←a1A1(0 0 0)] confirms infrared
Publikováno v:
Applied Physics B: Lasers and Optics. 76:467-471
The generation of programmable complex femtosecond pulses in the mid infrared (3–10 μm) with high precision is reported. Designed pulse shapes in the near infrared (1–1.6 μm) are transferred to the mid infrared via difference-frequency mixing w