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Directed evolution of non-heme iron enzymes to access abiological radical-relay C(sp(3))—H azidation
Autor:
Rui, Jinyan, Zhao, Qun, Huls, Anthony J., Soler, Jordi, Paris, Jared C., Chen, Zhenhong, Reshetnikov, Viktor, Yang, Yunfang, Guo, Yisong, Garcia-Borràs, Marc, Huang, Xiongyi
Publikováno v:
Science
We report here the reprogramming of non-heme iron enzymes to catalyze an abiological C(sp(3))—H azidation reaction via iron-catalyzed radical relay. This biocatalytic transformation uses amidyl radicals as hydrogen atom abstractors and Fe(III)—N(
Externí odkaz:
https://explore.openaire.eu/search/publication?articleId=pmid________::5e366af42048be23965234c39417e499
https://europepmc.org/articles/PMC9933208/
https://europepmc.org/articles/PMC9933208/
Akademický článek
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Autor:
Jinyan Rui, Qun Zhao, Huls, Anthony J., Soler, Jordi, Paris, Jared C., Zhenhong Chen, Reshetnikov, Viktor, Yunfang Yang, Yisong Guo, Garcia-Borràs, Marc, Xiongyi Huang
Publikováno v:
Science; 5/20/2022, Vol. 376 Issue 6595, p869-874, 6p, 4 Diagrams
Autor:
Zhang JG; Department of Chemistry, Johns Hopkins University; Baltimore, Maryland 21218, United States., Huls AJ; Department of Chemistry, Johns Hopkins University; Baltimore, Maryland 21218, United States., Palacios PM; Department of Chemistry, Carnegie Mellon University, Pittsburgh, Pennsylvania 15213, United States., Guo Y; Department of Chemistry, Carnegie Mellon University, Pittsburgh, Pennsylvania 15213, United States., Huang X; Department of Chemistry, Johns Hopkins University; Baltimore, Maryland 21218, United States.
Publikováno v:
Journal of the American Chemical Society [J Am Chem Soc] 2024 Dec 05. Date of Electronic Publication: 2024 Dec 05.