Reversible restructuring of supported Au nanoparticles during butadiene hydrogenation revealed by operando GISAXS/GIWAXS

Autor: James Martin, David, Decarolis, Donato, Odarchenko, Yaroslav I., Herbert, Jennifer J., Arnold, Thomas, Rawle, Jonathan, Nicklin, Chris, Boyen, Hans-Gerd, Beale, Andrew M.

Periodically arranged, monodisperse gold nanoparticles supported on flat silicon substrates were studied for the hydrogenation of 1,3-butadiene under operando conditions using Grazing Incidence Small- and Wide-Angle X-ray Scattering (GISAXS/GIWAXS).

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http://hdl.handle.net/1942/23676

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Reversible restructuring of supported Au nanoparticles during butadiene hydrogenation revealed by operando GISAXS/GIWAXS.

Autor: James Martin D; Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK. Andrew.Beale@ucl.ac.uk and Research Complex at Harwell (RCaH), Harwell, Didcot, Oxfordshire OX11 0FA, UK and Van't Hoff Institute for Molecular Sciences, University of Amsterdam, Amsterdam, 1098XH, Netherlands., Decarolis D; Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK. Andrew.Beale@ucl.ac.uk and Research Complex at Harwell (RCaH), Harwell, Didcot, Oxfordshire OX11 0FA, UK., Odarchenko YI; Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK. Andrew.Beale@ucl.ac.uk and Research Complex at Harwell (RCaH), Harwell, Didcot, Oxfordshire OX11 0FA, UK., Herbert JJ; Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK. Andrew.Beale@ucl.ac.uk and Research Complex at Harwell (RCaH), Harwell, Didcot, Oxfordshire OX11 0FA, UK and Netherlands Organisation for Scientific Research (NWO), DUBBLE CRG@ESRF, Grenoble 38042, France., Arnold T; Diamond Light Source, Harwell Science and Innovation Campus, Chilton, Didcot OX11 0DE, UK., Rawle J; Diamond Light Source, Harwell Science and Innovation Campus, Chilton, Didcot OX11 0DE, UK., Nicklin C; Diamond Light Source, Harwell Science and Innovation Campus, Chilton, Didcot OX11 0DE, UK., Boyen HG; Institute for Materials Research, Hasselt University, Diepenbeek, Belgium., Beale AM; Department of Chemistry, University College London, 20 Gordon Street, London, WC1H 0AJ, UK. Andrew.Beale@ucl.ac.uk and Research Complex at Harwell (RCaH), Harwell, Didcot, Oxfordshire OX11 0FA, UK.

Publikováno v: Chemical communications (Cambridge, England) [Chem Commun (Camb)] 2017 May 04; Vol. 53 (37), pp. 5159-5162.