Zobrazeno 1 - 8 of 8 pro vyhledávání: '"Gilles, De Smet"'
1
Access to Biorenewable and CO2-Based Polycarbonates from Exovinylene Cyclic Carbonates
Autor: Christophe Detrembleur, Connie Ocando, Julien De Winter, Bert U. W. Maes, Alejandro J. Müller, Bruno Grignard, Veronique Van Speybroeck, Elias Van Den Broeck, Gilles De Smet, Fabiana Siragusa
Publikováno v: ACS Sustainable Chemistry & Engineering. 9:1714-1728
We investigate the scope of the organocatalyzed step-growth copolymerization of CO2-sourced exovinylene bicyclic carbonates with bio-based diols into polycarbonates. A series of regioregular poly(oxo-carbonate)s were prepared from sugar- (1,4-butaned
Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_________::aad461bbaea1bfd63f431bdd307d8584
https://doi.org/10.1021/acssuschemeng.0c07683
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2
Homogeneous and heterogeneous catalysts for hydrogenation of CO2 to methanol under mild conditions
Autor: Bert U. W. Maes, Cheng Zhou, Bert F. Sels, Yuhe Liao, Gilles De Smet, Shao-Tao Bai, Matthias Beller, Ruiyan Sun
Publikováno v: Chemical Society Reviews. 50:4259-4298
In the context of a carbon neutral economy, catalytic CO2 hydrogenation to methanol is one crucial technology for CO2 mitigation providing solutions for manufacturing future fuels, chemicals, and materials. However, most of the presently known cataly
Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::3d253b9bac31ea4376784fc744a9779b
https://doi.org/10.1039/d0cs01331e
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3
Selective Nickel‐Catalyzed Hydrodeacetoxylation of Aryl Acetates
Autor: Gilles De Smet, Xingfeng Bai, Carl Mensch, Sergey Sergeyev, Gwilherm Evano, Bert U. W. Maes
Publikováno v: Angewandte Chemie: international edition in English
Acetate serves as a renewable and easily installed leaving group for selective deoxygenation of phenolics (ArOH). Ni-catalyzed hydrodeacetoxylation of aryl acetates (Ar-OAc) with HBpin in a green carbonate solvent selectively delivers the correspondi
Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::3ce103ac2bc7b80f4c2387578e2a35a0
https://doi.org/10.1002/anie.202201751
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5
Electrochemical quinuclidine-mediated C–H activation: Intermediates and mechanism
Autor: Filip Vorobjov, Gilles De Smet, Nick Daems, H.Y. Vincent Ching, Pieter Leveque, Bert U.W. Maes, Tom Breugelmans
Publikováno v: Journal of electroanalytical chemistry : an international journal devoted to all aspects of electrode kynetics, interfacial structure, properties of electrolytes, colloid and biological electrochemistry.
The reaction mechanism of quinuclidine mediated C-H oxidation of unactivated C-H bonds has been elucidated. In-situ cathodically generated H2O2 was shown to diffuse to the anode where it is oxidized and participates in the ketonization reaction. Furt
Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::06d3ca8674e2b7b14c10f43049898c46
https://doi.org/10.1016/j.jelechem.2022.116835
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6
Carbamate Synthesis Using a Shelf‐Stable and Renewable C 1 Reactant
Autor: Carl Mensch, Sergey Sergeyev, Charles Beromeo Bheeter, Bert U. W. Maes, Zoltán Dobi, Chen Chen, Gilles De Smet, Wouter A. Herrebout, B. Narendraprasad Reddy, Laurent Van Raemdonck, Evelien Renders
Publikováno v: Chemsuschem
4-Propylcatechol carbonate is a shelf-stable, renewable C1 reactant. It is easily prepared from renewable 4-propylcatechol (derived from wood) and dimethyl carbonate (derived from CO2 ) using a reactive distillation system. In this work, the 4-propyl
Externí odkaz: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::5629621e51e039f719ea2238c2b7adff
https://doi.org/10.1002/cssc.201900406
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