Zobrazeno 1 - 10
of 86
pro vyhledávání: '"Gerd, Kothe"'
Autor:
Gerd Kothe, Konstantin L. Ivanov, Michail Lukaschek, Tomoaki Yago, Gerhard Link, Tien-Sung Lin
Publikováno v:
The Journal of Physical Chemistry Letters. 12:3647-3654
Quantum entanglement has been realized on a variety of physical platforms such as quantum dots, trapped atomic ions, and superconductors. Here we introduce specific molecular solids as promising alternative platforms. Our model system is triplet pent
Autor:
Gerd, Kothe, Michail, Lukaschek, Tomoaki, Yago, Gerhard, Link, Konstantin L, Ivanov, Tien-Sung, Lin
Publikováno v:
The journal of physical chemistry letters. 12(14)
Quantum entanglement has been realized on a variety of physical platforms such as quantum dots, trapped atomic ions, and superconductors. Here we introduce specific molecular solids as promising alternative platforms. Our model system is triplet pent
Autor:
Boris Illarionov, Wolfgang Eisenreich, Monika Joshi, Gerd Kothe, Adelbert Bacher, Stefan Weber, Michail Lukaschek, Nediljko Budisa, Markus Fischer, Sylwia Kacprzak
Publikováno v:
The Journal of Physical Chemistry B. 119:13934-13943
The photo-CIDNP effect has proven to be useful to strongly enhance NMR signals of photochemically active proteins simply by irradiation with light. The evolving characteristic patterns of enhanced absorptive and emissive NMR lines can be exploited to
Autor:
Patricia Stehle, Christoph F. Beck, Gerhard Link, Gerd Kothe, Oleg G. Poluektov, Erika Donner von Gromoff, Peter Heathcote, Thomas Berthold, Stefano Santabarbara, Marion C. Thurnauer
Publikováno v:
Journal of the American Chemical Society. 134:5563-5576
Crystallographic models of photosystem I (PS I) highlight a symmetrical arrangement of the electron transfer cofactors which are organized in two parallel branches (A, B) relative to a pseudo-C2 symmetry axis that is perpendicular to the membrane pla
Autor:
Gerhard Link, Michail Lukaschek, Tien-Sung Lin, Gerd Kothe, Jörg-Ulrich Weidner, Tomoaki Yago
Publikováno v:
The Journal of Physical Chemistry B. 114:14755-14762
The unique physical properties of photoexcited triplet states have been explored in numerous spectroscopic studies employing electron paramagnetic resonance (EPR). So far, however, no quantum interference effects were found in these systems in the pr
Autor:
Marion C. Thurnauer, Gerd Kothe
Publikováno v:
Photosynthesis Research. 102:349-365
The primary energy conversion steps of natural photosynthesis proceed via light-induced radical ion pairs as short-lived intermediates. Time-resolved electron paramagnetic resonance (EPR) experiments of photosynthetic reaction centers monitor the key
Publikováno v:
Chemical Physics Letters. 438:351-357
Using the density operator formalism, an analytical model is developed to study the time evolution of the electron spin magnetization of photo-excited triplet states in an external magnetic field. Analysis reveals that pulsed light excitation initiat
Autor:
Gerd Kothe, Zeev Gross, Haim Levanon, Liliya Simkhovich, Thomas Berthold, Israel Goldberg, Eli Stavitski, Linn Wagnert, Alexander Berg, Atif Mahammed
Publikováno v:
Applied Magnetic Resonance. 30:591-604
The photoexcited triplet states of three 5,10, 15-tris(pentafluorophenyl)corroles (tpfc), hosting Sn(IV) and Al(III) in their core, namely, Sn(Cl)(tpfc), Al(pyr)2(tpfc) and Al(pyr)2(tpfc-Br8), were studied by time-resolved electron paramagnetic reson
Publikováno v:
The Journal of Physical Chemistry B. 108:9505-9515
The analysis of the influence of director fluctuations on the ESR spectra of a spin probe dissolved in oriented phases (liquid crystals, membranes) requires a slow-motional treatment because the director field has always slowly relaxing components. T
Autor:
Sandra L. Schlesselman, Thomas Berthold, Diego Frezzato, Oleg G. Poluektov, Ernst Ohmes, U. Heinen, Gerd Kothe, Giorgio J. Moro, J. R. Golecki, Marion C. Thurnauer
Publikováno v:
Applied Magnetic Resonance. 26:99-115
Spin-correlated radical pairs are the short-lived intermediates of the primary energy conversion steps of photosynthesis. In this paper, we develop a comprehensive model for the spin-polarized electron paramagnetic resonance (EPR) spectra of these sy