Zobrazeno 1 - 10
of 31
pro vyhledávání: '"Frank Garisto"'
Autor:
Robert J. Lemire, Frank Garisto
Publikováno v:
ract. :37-52
Autor:
N. C. Garisto, Frank Garisto
Publikováno v:
Annals of Nuclear Energy. 17:183-193
Bentonite-based clays are proposed as a barrier to radionuclide migration in the geological disposal of used UO2 fuel. There is some evidence, however, that this buffer may be susceptible to cracking. Therefore, we have investigated the effect of cra
Autor:
Raymond Kapral, Frank Garisto
Publikováno v:
The Journal of Chemical Physics. 64:3826-3832
In this article the results of a fairly extensive set of mode coupling calculations of both the anomalous Rayleigh linewidth and shear viscosity of xenon are presented. The trilinear kinetic equations for the order parameter fluctuations are presente
Autor:
Frank Garisto
Publikováno v:
Annals of Nuclear Energy. 16:33-38
α-radiolysis could affect the dissolution behaviour of used UO2 fuel. To model this effect, one must first determine the α-radiation dose absorbed by the water near the fuel surface, e.g. in fuel cracks. This is the purpose of our paper. First, usi
Publikováno v:
The Journal of Chemical Physics. 79:6294-6300
The solvation energy of hard spherical ions immersed in dipolar hard sphere solvents is investigated as a function of ion diameter. We apply both the mean spherical and linearized hypernetted‐chain approximations and show that for ions of physicall
Autor:
N. C. Garisto, Frank Garisto
Publikováno v:
Nuclear and Chemical Waste Management. 6:203-211
The oxidative dissolution of UO2 has been stimulated using thermodynamic reaction-path calculations. The extent of dissolution (as a function of the reaction coordinate) and the solid oxidation sequences are reported for various pH values, ligand (ca
Autor:
N. C. Garisto, Frank Garisto
Publikováno v:
Nuclear Science and Engineering. 90:103-110
An explicit mathematical formula has been derived, using thermodynamic principles, for the calculation of uranium dioxide solubilities as a function of temperature, pH, oxidation potential, and anion (carbonate, phosphate, sulfate, or chloride) conce
Autor:
Frank Garisto, Raymond Kapral
Publikováno v:
Physical Review A. 10:309-318
Autor:
G. N. Patey, Frank Garisto
Publikováno v:
Chemical Physics Letters. 117:457-460
In dilute ionic solutions, the solute-dependent dielectric constant varies as a linear function of concentration. In this note we consider alternative theoretical routes to the limiting slope, and compare numerical results for ions in dipolar hard-sp