Zobrazeno 1 - 10
of 59
pro vyhledávání: '"Dennis E. Sparks"'
Publikováno v:
Catalysis Today. 343:137-145
Deuterium tracer studies coupled with kinetic approach were developed to accurately determine the kinetic isotopic effects (KIE) for the CO hydrogenation and the formations of CO2, CH4 and light hydrocarbons (C2-C4) over iron, cobalt and ruthenium ca
Autor:
Wenping Ma, Burtron H. Davis, Dennis E. Sparks, Dragomir B. Bukur, Gary Jacobs, Branislav Todic
Publikováno v:
Catalysis Today
Quantitative data comparing iron and cobalt based catalysts for the Fischer-Tropsch synthesis (FTS) are scarce due to the fact that these two kinds of catalysts typically utilize different process conditions. This paper focuses on studying the cataly
Autor:
Muthu Kumaran Gnanamani, Michela Martinelli, Shelley D. Hopps, Dennis E. Sparks, Aimee MacLennan, Gary Jacobs, Burtron H. Davis, Yongfeng Hu
Publikováno v:
ChemCatChem. 10:3709-3716
Autor:
Jia Yang, Hussein H. Hamdeh, Dennis E. Sparks, Wenping Ma, Gary Jacobs, Burtron H. Davis, Wilson D. Shafer
Publikováno v:
Applied Catalysis A: General. 560:144-152
The explanation for CH4 selectivity for iron based Fischer-Tropsch catalysts in the low conversion region (i.e.
Fischer-Tropsch synthesis. Effect of KCl contaminant on the performance of iron and cobalt catalysts
Autor:
Gerald A. Thomas, Venkat Ramana Rao Pendyala, Burtron H. Davis, Yongfeng Hu, Aimee MacLennan, Dennis E. Sparks, Wenping Ma, Gary Jacobs, Wilson D. Shafer
Publikováno v:
Catalysis Today. 299:28-36
As a follow-up to a previous alkali chloride poisoning study, the effect of up to 100 ppm KCl on the Fischer-Tropsch synthesis (FTS) performance of representative iron (Fe-Si-Cu doped with Rb as the alkali) and cobalt (Pt-Co/Al 2 O 3 ) catalysts was
Autor:
Michela Martinelli, Gary Jacobs, Venkat Ramana Rao Pendyala, Burtron H. Davis, Wilson D. Shafer, Dennis E. Sparks
Publikováno v:
RSC Advances. 7:7793-7800
The effects of co-fed ammonia in synthesis gas on the activity and product selectivities of a typical cobalt catalyst (0.5% Pt–25% Co/Al2O3) were investigated during the Fischer–Tropsch synthesis using a continuously stirred tank reactor (CSTR).
Publikováno v:
Faraday Discuss.. 197:403-419
Fischer-Tropsch synthesis was conducted in a small channel compact heat exchange reactor that was constructed of aluminum. While limited to lower temperature-pressure regions of the Fischer-Tropsch synthesis, the reactor could be operated in an isoth
Autor:
Chia H. Yen, Gary Jacobs, Jennifer L.S. Klettlinger, Burtron H. Davis, Dennis E. Sparks, Wenping Ma
Publikováno v:
Catalysis Today. 275:49-58
A large number of kinetic data points (83 sets) was obtained over a wide range of CO conversion (7–90%), pressure (1.3–2.5 MPa) and H 2 /CO ratio (0.67–1.5) with an iron catalyst (100 Fe/5.1 Si/1.25 K). The kinetics of the catalyst in the low (
Autor:
Venkat Ramana Rao Pendyala, Gerald A. Thomas, Muthu Kumaran Gnanamani, Qunfeng Xiao, Burtron H. Davis, Dennis E. Sparks, Yongfeng Hu, Shelley D. Hopps, Wilson D. Shafer, Gary Jacobs, Uschi M. Graham
Publikováno v:
Applied Catalysis A: General. 523:146-158
The effect of phosphorus addition on silica-supported cobalt catalyst was investigated for Fischer-Tropsch synthesis (FTS). As shown by STEM images and chemisorption, the addition of phosphorus to cobalt of up to 1 wt% increased the dispersion of cob
Autor:
Qunfeng Xiao, Dennis E. Sparks, Yongfeng Hu, Wilson D. Shafer, Burtron H. Davis, Venkat Ramana Rao Pendyala, Syed Khalid, Gary Jacobs, Wenping Ma
Publikováno v:
Catalysis Letters. 146:1858-1866
The effect of co-fed hydrogen chloride (HCl) in syngas on the performance of iron and cobalt-based Fischer–Tropsch (FT) catalysts was investigated in our earlier studies (Ma et al. in ACS Catal 5:3124–3136, 2015; Davis et al., DOE final report, 2