Zobrazeno 1 - 7
of 7
pro vyhledávání: '"Constantin Heshmatpour"'
Autor:
Andreas V. Stier, Jonathan J. Finley, Jürgen Hauer, Dario Polli, Antonio Perri, Erling Thyrhaug, Constantin Heshmatpour, Lukas Wolz, Giulio Cerullo
Publikováno v:
Review of Scientific Instruments
We present diffraction-limited photocurrent (PC) microscopy in the visible spectral range based on broadband excitation and an inherently phase-stable common-path interferometer. The excellent path-length stability guarantees high accuracy without th
Autor:
Christoph Lambert, Constantin Heshmatpour, František Šanda, Felix Plasser, Pavel Malevich, Jürgen Hauer, Maximilian F. S. J. Menger
Publikováno v:
JOURNAL OF PHYSICAL CHEMISTRY LETTERS, 11(18), 7776-7781. AMER CHEMICAL SOC
Exciton-exciton annihilation (EEA) is a ubiquitous phenomenon, which may limit the efficiency of photovoltaic devices. Conventional methods of determining EEA time scales rely on measuring the intensity dependence of third-order signals. In this work
Publikováno v:
The 22nd International Conference on Ultrafast Phenomena 2020.
We present a fully non-collinear 50 kHz shot-to-shot detected two-dimensional electronic spectroscopy setup for directly studying bi-exciton relaxation dynamics via 5th order signals. The measurements report on annihilation timescales at a single, pe
Publikováno v:
The Journal of Chemical Physics. 156:084114
Correlated spectral fluctuations were suggested to coordinate excitation transport inside natural light harvesting complexes. We demonstrate the capacities of 2D line shapes from fifth-order coherent electronic signals (R5-2D) to report on such fluct
Autor:
Jürgen Hauer, Maximilian H. Schreck, Harald Ceymann, Constantin Heshmatpour, Craig N. Lincoln, Pavel Malevich
Publikováno v:
EPJ Web of Conferences, Vol 205, p 06013 (2019)
We present 5th and 3rd order 2D spectra of a squarine trimer. Slowly decaying (τ = 0.8 ps) and intensity dependent features unique to the 5th order signal are attributed to exciton-exciton annihilation.
Autor:
Jürgen Hauer, Pavel Malevich, František Šanda, Craig N. Lincoln, Václav Perlík, Constantin Heshmatpour
Publikováno v:
EPJ Web of Conferences, Vol 205, p 06016 (2019)
We present simulations of 3rd and 5th order multidimensional time-dependent signals of a molecular trimer. The developed model allows for the simulation of both signal types within one theoretical framework. We therefore extended standard Redfield th
Publikováno v:
Chemical Physics. 528:110433
Multidimensional fifth order spectroscopy is a sophisticated and specialized tool for probing bi-exciton dynamics. The complexity of the signals emitted into ± 2 K → 1 ∓ 2 K → 2 + K → 3 directions calls for a detailed theoretical treatment o