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An experimental and computational study of CO2adsorption in the sodalite-type M-BTT (M = Cr, Mn, Fe, Cu) metal-organic frameworks featuring open metal sites

Autor: Asgari, M, Jawahery, S, Bloch, ED, Hudson, MR, Flacau, R, Vlaisavljevich, B, Long, JR, Brown, CM, Queen, WL

Publikováno v: Asgari, M; Jawahery, S; Bloch, ED; Hudson, MR; Flacau, R; Vlaisavljevich, B; et al.(2018). An experimental and computational study of CO2adsorption in the sodalite-type M-BTT (M = Cr, Mn, Fe, Cu) metal-organic frameworks featuring open metal sites. Chemical Science, 9(20), 4579-4588. doi: 10.1039/c8sc00971f. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/4kw9k14d

© 2018 The Royal Society of Chemistry. We present a comprehensive investigation of the CO2adsorption properties of an isostructural series of metal-organic frameworks, M-BTT (M = Cr, Mn, Fe, Cu; BTT3-= 1,3,5-benzenetristetrazolate), which exhibit a

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Structural characterization of framework-gas interactions in the metal-organic framework Co2(dobdc) by: In situ single-crystal X-ray diffraction

Autor: Gonzalez, MI, Mason, JA, Bloch, ED, Teat, SJ, Gagnon, KJ, Morrison, GY, Queen, WL, Long, JR

Publikováno v: Gonzalez, MI; Mason, JA; Bloch, ED; Teat, SJ; Gagnon, KJ; Morrison, GY; et al.(2017). Structural characterization of framework-gas interactions in the metal-organic framework Co2(dobdc) by: In situ single-crystal X-ray diffraction. Chemical Science, 8(6), 4387-4398. doi: 10.1039/c7sc00449d. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/45k3b7mf

© 2017 The Royal Society of Chemistry. The crystallographic characterization of framework-guest interactions in metal-organic frameworks allows the location of guest binding sites and provides meaningful information on the nature of these interactio

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Critical Factors Driving the High Volumetric Uptake of Methane in Cu3(btc)2

Autor: Hulvey, Z, Vlaisavljevich, B, Mason, JA, Tsivion, E, Dougherty, TP, Bloch, ED, Head-Gordon, M, Smit, B, Long, JR, Brown, CM

Publikováno v: Hulvey, Z; Vlaisavljevich, B; Mason, JA; Tsivion, E; Dougherty, TP; Bloch, ED; et al.(2015). Critical Factors Driving the High Volumetric Uptake of Methane in Cu3(btc)2. Journal of the American Chemical Society, 137(33), 10816-10825. doi: 10.1021/jacs.5b06657. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/8qn2g5n6

© 2015 American Chemical Society. A thorough experimental and computational study has been carried out to elucidate the mechanistic reasons for the high volumetric uptake of methane in the metal-organic framework Cu3(btc)2 (btc3- = 1,3,5-benzenetric

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Cooperative insertion of CO2in diamine-appended metal-organic frameworks

Publikováno v: McDonald, TM; Mason, JA; Kong, X; Bloch, ED; Gygi, D; Dani, A; et al.(2015). Cooperative insertion of CO2in diamine-appended metal-organic frameworks. Nature, 519(7543), 303-308. doi: 10.1038/nature14327. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/2vs0h0wg

© 2015 Macmillan Publishers Limited. The process of carbon capture and sequestration has been proposed as a method of mitigating the build-up of greenhouse gases in the atmosphere. If implemented, the cost of electricity generated by a fossil fuel-b

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NMR relaxation and exchange in metal-organic frameworks for surface area screening

Autor: Chen, JJ, Mason, JA, Bloch, ED, Gygi, D, Long, JR, Reimer, JA

Publikováno v: Chen, JJ; Mason, JA; Bloch, ED; Gygi, D; Long, JR; & Reimer, JA. (2015). NMR relaxation and exchange in metal-organic frameworks for surface area screening. Microporous and Mesoporous Materials, 205, 65-69. doi: 10.1016/j.micromeso.2014.07.037. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/3pv7410j

© 2014 Elsevier Inc.All rights reserved. We describe a robust screening technique that correlates the surface area of metal-organic frameworks to the proton T2relaxation behavior of imbibed solvent at low field (13 MHz). In frameworks with small por

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Selective propene oligomerization with nickel(II)-based metal-organic frameworks

Autor: Mlinar, AN, Keitz, BK, Gygi, D, Bloch, ED, Long, JR, Bell, AT

Publikováno v: ACS Catalysis, vol 4, iss 3
Mlinar, AN; Keitz, BK; Gygi, D; Bloch, ED; Long, JR; & Bell, AT. (2014). Selective propene oligomerization with nickel(II)-based metal-organic frameworks. ACS Catalysis, 4(3), 717-721. doi: 10.1021/cs401189a. UC Berkeley: Retrieved from: http://www.escholarship.org/uc/item/96g0r90f

Two Ni2+-containing metal-organic frameworks, Ni 2(dobdc) and Ni2(dobpdc), are shown to be active for the oligomerization of propene in the gas phase. The metal-organic frameworks exhibit activity comparable to Ni2+-exchanged aluminosilicates but mai

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