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Temporal reversibility of reactive systems out of equilibrium: A strange paradox

Autor: Politano, O., Garcia, Alejandro L., Baras, F., Mansour, M. Malek

The second law of thermodynamics stipulates that entropy production is non-negative in macroscopic systems, reaching zero at thermodynamic equilibrium. As a corollary, this implies that the state trajectory of macroscopic systems is inherently time-i

Externí odkaz: http://arxiv.org/abs/2410.19578

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Reply to 'Comment on `Validity of path thermodynamic description of reactive systems: Microscopic simulations'

Autor: Baras, F., Garcia, A. L., Mansour, M. Malek

The Comment's author argues that a correct description of reactive systems should incorporate the explicit interaction with reservoirs, leading to a unified system-reservoirs entity. However, this proposition has two major flaws. Firstly, as we will

Externí odkaz: http://arxiv.org/abs/2309.05485

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Validity of path thermodynamic description of reactive systems: Microscopic simulations

Autor: Baras, F., Garcia, A. L., Mansour, M. Malek

Traditional stochastic modeling of reactive systems limits the domain of applicability of the associated path thermodynamics to systems involving a single elementary reaction at the origin of each observed change in composition. An alternative stocha

Externí odkaz: http://arxiv.org/abs/2210.01952

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